Bands, resonances, edge singularities and excitons in core level spectroscopy investigated within the dynamical mean-field theory

Using a recently developed impurity solver we exemplify how dynamical mean-field theory captures band excitations, resonances, edge singularities and excitons in core level x-ray absorption spectroscopy (XAS) and core level photo electron spectroscopy (cPES) on metals, correlated metals and Mott ins...

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Hauptverfasser: Haverkort, Maurits W. (VerfasserIn) , Lu, Yi (VerfasserIn)
Dokumenttyp: Article (Journal)
Sprache:Englisch
Veröffentlicht: 5 December 2014
In: epl
Year: 2014, Jahrgang: 108, Heft: 5, Pages: 57004
ISSN:1286-4854
DOI:10.1209/0295-5075/108/57004
Online-Zugang:Verlag, Volltext: http://dx.doi.org/10.1209/0295-5075/108/57004
Verlag, Volltext: http://stacks.iop.org/0295-5075/108/i=5/a=57004
Volltext
Verfasserangaben:M. W. Haverkort, G. Sangiovanni, P. Hansmann, A. Toschi, Y. Lu, and S. Macke
Beschreibung
Zusammenfassung:Using a recently developed impurity solver we exemplify how dynamical mean-field theory captures band excitations, resonances, edge singularities and excitons in core level x-ray absorption spectroscopy (XAS) and core level photo electron spectroscopy (cPES) on metals, correlated metals and Mott insulators. Comparing XAS at different values of the core-valence interaction shows how the quasiparticle peak in the absence of core-valence interactions evolves into a resonance of similar shape, but different origin. Whereas XAS is rather insensitive to the metal insulator transition, cPES can be used, due to nonlocal screening, to measure the amount of local charge fluctuation.
Beschreibung:Gesehen am 27.09.2017
Beschreibung:Online Resource
ISSN:1286-4854
DOI:10.1209/0295-5075/108/57004