Photoelectron spin-polarization control in the topological insulator Bi 2Se 3

We study the manipulation of the spin polarization of photoemitted electrons in Bi2Se3 by spin- and angle-resolved photoemission spectroscopy. General rules are established that enable controlling the photoelectron spin-polarization. We demonstrate the ± 100% reversal of a single component of the me...

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Hauptverfasser: Zhu, Zheng H. (VerfasserIn) , Veenstra, C. N. (VerfasserIn) , Haverkort, Maurits W. (VerfasserIn)
Dokumenttyp: Article (Journal)
Sprache:Englisch
Veröffentlicht: 20 February 2014
In: Physical review letters
Year: 2014, Jahrgang: 112, Heft: 7, Pages: 076802
ISSN:1079-7114
DOI:10.1103/PhysRevLett.112.076802
Online-Zugang:Verlag, Volltext: http://dx.doi.org/10.1103/PhysRevLett.112.076802
Verlag, Volltext: https://link.aps.org/doi/10.1103/PhysRevLett.112.076802
Volltext
Verfasserangaben:Z.-H. Zhu, C.N. Veenstra, S. Zhdanovich, M.P. Schneider, T. Okuda, K. Miyamoto, S.-Y. Zhu, H. Namatame, M. Taniguchi, M.W. Haverkort, I.S. Elfimov, and A. Damascelli

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520 |a We study the manipulation of the spin polarization of photoemitted electrons in Bi2Se3 by spin- and angle-resolved photoemission spectroscopy. General rules are established that enable controlling the photoelectron spin-polarization. We demonstrate the ± 100% reversal of a single component of the measured spin-polarization vector upon the rotation of light polarization, as well as full three-dimensional manipulation by varying experimental configuration and photon energy. While a material-specific density-functional theory analysis is needed for the quantitative description, a minimal yet fully generalized two-atomic-layer model qualitatively accounts for the spin response based on the interplay of optical selection rules, photoelectron interference, and topological surface-state complex structure. It follows that photoelectron spin-polarization control is generically achievable in systems with a layer-dependent, entangled spin-orbital texture. 
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