Determination of the orbital moment and crystal field splitting in LaTiO3
Utilizing a sum-rule in a spin-resolved photoelectron spectroscopic experiment with circularly polarized light, we show that the orbital moment in LaTiO$_3$ is strongly reduced both below and above the N\'{e}el temperature. Using Ti $L_{2,3}$ x-ray absorption spectroscopy as a local probe, we f...
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| Dokumenttyp: | Article (Journal) Kapitel/Artikel |
| Sprache: | Englisch |
| Veröffentlicht: |
2004
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| In: |
Arxiv
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| Online-Zugang: | Verlag, kostenfrei, Volltext: http://arxiv.org/abs/astro-ph/0405516
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| Verfasserangaben: | M.W. Haverkort, Z. Hu, A. Tanaka, G. Ghiringhelli, H. Roth, M. Cwik, T. Lorenz, C. Schuessler-Langeheine, S.V. Streltsov, A.S. Mylnikova, V.I. Anisimov, C. de Nadai, N.B. Brookes, H.H. Hsieh, H.-J. Lin, C.T. Chen, T. Mizokawa, Y. Taguchi, Y. Tokura, D.I. Khomskii, and L.H. Tjeng |
| Zusammenfassung: | Utilizing a sum-rule in a spin-resolved photoelectron spectroscopic experiment with circularly polarized light, we show that the orbital moment in LaTiO$_3$ is strongly reduced both below and above the N\'{e}el temperature. Using Ti $L_{2,3}$ x-ray absorption spectroscopy as a local probe, we found that the crystal field splitting in the $t_{2g}$ subshell is about 0.12-0.30 eV. This large splitting does not facilitate the formation of an orbital liquid. |
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| Beschreibung: | Im Titel ist "3" tiefgestellt Gesehen am 28.11.2017 |
| Beschreibung: | Online Resource |