Anisotropy-governed competition of magnetic phases in the honeycomb quantum magnet Na3Ni2SbO6 studied by dilatometry and high-frequency ESR
Thermodynamic properties and low-energy magnon excitations of S=1 honeycomb-layered Na3Ni2SbO6 have been investigated by high-resolution dilatometry, static magnetization, and high-frequency electron spin resonance studies in magnetic fields up to 16 T. At TN = 16.5 K, there is a tricritical point s...
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| Main Authors: | , , , , , |
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| Format: | Article (Journal) |
| Language: | English |
| Published: |
20 June 2017
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| In: |
Physical review
Year: 2017, Volume: 95, Issue: 21 |
| ISSN: | 2469-9969 |
| DOI: | 10.1103/PhysRevB.95.214414 |
| Online Access: | Verlag, Volltext: http://dx.doi.org/10.1103/PhysRevB.95.214414 Verlag, Volltext: https://link.aps.org/doi/10.1103/PhysRevB.95.214414 
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| Author Notes: | J. Werner, W. Hergett, M. Gertig, J. Park, C. Koo, and R. Klingeler |
MARC
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| 245 | 1 | 0 | |a Anisotropy-governed competition of magnetic phases in the honeycomb quantum magnet Na3Ni2SbO6 studied by dilatometry and high-frequency ESR |c J. Werner, W. Hergett, M. Gertig, J. Park, C. Koo, and R. Klingeler |
| 246 | 3 | 3 | |a Anisotropy-governed competition of magnetic phases in the honeycomb quantum magnet Na 3 Ni 2 SbO 6 |
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| 520 | |a Thermodynamic properties and low-energy magnon excitations of S=1 honeycomb-layered Na3Ni2SbO6 have been investigated by high-resolution dilatometry, static magnetization, and high-frequency electron spin resonance studies in magnetic fields up to 16 T. At TN = 16.5 K, there is a tricritical point separating two distinct antiferromagnetic phases, AF1 and AF2, from the paramagnetic regime. In addition, our data imply short-range antiferromagnetic correlations at least up to ∼5TN. Well below TN, the magnetic field BC1≈9.5 T is needed to stabilize AF2 against AF1. The thermal expansion and magnetostriction anomalies at TN and BC1 imply significant magnetoelastic coupling, both of which are associated with a sign change of ∂L/∂B. The transition at BC1 is associated with softening of the antiferromagnetic resonance modes observed in the electron-spin-resonance spectra. The anisotropy gap Δ=360 GHz implies considerable uniaxial anisotropy. We deduce the crucial role of axial anisotropy favoring the AF1 spin structure over the AF2 one. While the magnetostriction data disprove a simple spin-flop scenario at BC1, the nature of a second transition at BC2 ≈ 13 T remains unclear. Both the sign of the magnetostriction and Grüneisen analysis suggest that the short-range correlations at high temperatures are of AF2 type. | ||
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