A comprehensive study of Interatomic Coulombic Decay in argon dimers: extracting R-dependent absolute decay rates from the experiment

In this work we present a comprehensive and detailed study of Interatomic Coulombic Decay (ICD) occurring after irradiating argon dimers with XUV-synchrotron radiation. A manifold of different decay channels is observed and the corresponding initial and final states are assigned. Additionally, the e...

Descripción completa

Guardado en:
Detalles Bibliográficos
Autores principales: Rist, Jonas (Autor) , Miteva, Tsveta (Autor) , Gokhberg, Kirill (Autor)
Formato: Article (Journal)
Lenguaje:inglés
Publicado: 2017
In: Chemical physics
Year: 2016, Volumen: 482, Pages: 185-191
DOI:10.1016/j.chemphys.2016.09.024
Acceso en línea:Verlag, Volltext: http://dx.doi.org/10.1016/j.chemphys.2016.09.024
Verlag, Volltext: http://www.sciencedirect.com/science/article/pii/S030101041630581X
Enlace del recurso
Notas de Autor:J. Rist, T. Miteva, B. Gaire, H. Sann, F. Trinter, M. Keiling, N. Gehrken, A. Moradmand, B. Berry, M. Zohrabi, M. Kunitski, I. Ben-Itzhak, A. Belkacem, T. Weber, A.L. Landers, M. Schöffler, J.B. Williams, P. Kolorenč, K. Gokhberg, T. Jahnke, R. Dörner
Descripción
Sumario:In this work we present a comprehensive and detailed study of Interatomic Coulombic Decay (ICD) occurring after irradiating argon dimers with XUV-synchrotron radiation. A manifold of different decay channels is observed and the corresponding initial and final states are assigned. Additionally, the effect of nuclear dynamics on the ICD electron spectrum is examined for one specific decay channel. The internuclear distance-dependent width Γ(R) of the decay is obtained from the measured kinetic energy release distribution of the ions employing a classical nuclear dynamics model.
Notas:Available online 15 September 2016
Gesehen am 27.06.2018
Descripción Física:Online Resource
DOI:10.1016/j.chemphys.2016.09.024