Kinetic energy release in fragmentation processes following electron emission: a time-dependent approach
A time-dependent approach for the kinetic energy release (KER) spectrum is developed for a fragmentation of a diatomic molecule after an electronic decay process, e.g., Auger process. It allows one to simulate the time-resolved spectra and provides more insight into the molecular dynamics than the t...
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| Hauptverfasser: | , , , |
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| Dokumenttyp: | Article (Journal) |
| Sprache: | Englisch |
| Veröffentlicht: |
19 March 2012
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| In: |
The journal of chemical physics
Year: 2012, Jahrgang: 136, Heft: 11, Pages: 1-12 |
| ISSN: | 1089-7690 |
| DOI: | 10.1063/1.3694536 |
| Online-Zugang: | Verlag, Volltext: http://dx.doi.org/10.1063/1.3694536 Verlag, Volltext: https://aip.scitation.org/doi/10.1063/1.3694536 
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| Verfasserangaben: | Ying-Chih Chiang, Frank Otto, Hans-Dieter Meyer and Lorenz S. Cederbaum |
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| 520 | |a A time-dependent approach for the kinetic energy release (KER) spectrum is developed for a fragmentation of a diatomic molecule after an electronic decay process, e.g., Auger process. It allows one to simulate the time-resolved spectra and provides more insight into the molecular dynamics than the time-independent approach. Detailed analysis of the time-resolved emitted electron and KER spectra sheds light on the interrelation between wave packet dynamics and spectra. | ||
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