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Dinuclear copper(II) complexes with distant metal centers: weaker donor groups increase catecholase activity

Two dinuclear complexes with Cu···Cu distances above 7 Å were characterized by X-ray diffraction, EPR spectroscopy, solution speciation, and cyclic voltammetry. Both complexes display EPR spectra typical of dipole-dipole-coupled dicopper(II) complexes. The two complexes presented herein are part of...

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Hauptverfasser: Zerón, Paulino (VerfasserIn) , Westphal, Michael (VerfasserIn) , Comba, Peter (VerfasserIn)
Dokumenttyp: Article (Journal)
Sprache:Englisch
Veröffentlicht: 2017
In: European journal of inorganic chemistry
Year: 2016, Heft: 1, Pages: 56-62
ISSN:1099-0682
DOI:10.1002/ejic.201600967
Online-Zugang:Verlag, Volltext: http://dx.doi.org/10.1002/ejic.201600967
Verlag, Volltext: https://onlinelibrary.wiley.com/doi/abs/10.1002/ejic.201600967
Volltext
Verfasserangaben:Paulino Zerón, Michael Westphal, Peter Comba, Marcos Flores‐Álamo, A. Claudia Stueckl, Carmen Leal‐Cervantes, Víctor M. Ugalde‐Saldívar, and Laura Gasque

MARC

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520 |a Two dinuclear complexes with Cu···Cu distances above 7 Å were characterized by X-ray diffraction, EPR spectroscopy, solution speciation, and cyclic voltammetry. Both complexes display EPR spectra typical of dipole-dipole-coupled dicopper(II) complexes. The two complexes presented herein are part of a series of dinuclear complexes with catecholase activity, and they exhibit the highest catalytic efficiencies of the series. This is associated with the weaker donor character of the ligands. 
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