Hot carrier relaxation in CdTe via phonon-plasmon modes

Carrier and lattice dynamics of laser excited CdTe was studied by time-resolved reflectivity for excitation fluences spanning about three orders of magnitude, from 0.064 to 6.14 mJ cm −2 . At fluences below 1 mJ cm −2 the transient reflectivity is dominated by the dynamics of hybrid phonon-plasmon m...

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Main Authors: Zhong, Yinpeng (Author) , Schlichting, Ilme (Author)
Format: Article (Journal)
Language:English
Published: 23 January 2017
In: Journal of physics. Condensed matter
Year: 2017, Volume: 29, Issue: 9
ISSN:1361-648X
DOI:10.1088/1361-648X/aa5478
Online Access:Verlag, Volltext: http://dx.doi.org/10.1088/1361-648X/aa5478
Verlag, Volltext: http://stacks.iop.org/0953-8984/29/i=9/a=095701
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Author Notes:Y. Zhong, D. Ostach, M. Scholz, S.W. Epp, S. Techert, I. Schlichting, J. Ullrich, F.S. Krasniqi

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520 |a Carrier and lattice dynamics of laser excited CdTe was studied by time-resolved reflectivity for excitation fluences spanning about three orders of magnitude, from 0.064 to 6.14 mJ cm −2 . At fluences below 1 mJ cm −2 the transient reflectivity is dominated by the dynamics of hybrid phonon-plasmon modes. At fluences above 1 mJ cm −2 the time-dependent reflectivity curves show a complex interplay between band-gap renormalization, band filling, carrier dynamics and recombination. A framework that accounts for such complex dynamics is presented and used to model the time-dependent reflectivity data. This model suggests that the excess energy of the laser-excited hot carriers is reduced much more efficiently by emitting hybrid phonon-plasmon modes rather than bare longitudinal optical phonons. 
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