Full characterization of the third-order nonlinear susceptibility using a single-beam coherent anti-Stokes Raman scattering setup
A method for the full determination of the third-order nonlinear coherent anti-Stokes Raman scattering (CARS) susceptibility is presented, which relies on phase control of a single ultrabroadband femtosecond laser pulse. A narrowband phase gate is scanned to perform double quadrature spectral interf...
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| Hauptverfasser: | , , , |
|---|---|
| Dokumenttyp: | Article (Journal) |
| Sprache: | Englisch |
| Veröffentlicht: |
October 9, 2012
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| In: |
Optics letters
Year: 2012, Jahrgang: 37, Heft: 20, Pages: 4239-4241 |
| ISSN: | 1539-4794 |
| DOI: | 10.1364/OL.37.004239 |
| Online-Zugang: | Verlag, Volltext: http://dx.doi.org/10.1364/OL.37.004239 Verlag, Volltext: https://www.osapublishing.org/ol/abstract.cfm?uri=ol-37-20-4239 
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| Verfasserangaben: | Alexander Wipfler, Jean Rehbinder, Tiago Buckup, and Marcus Motzkus |
MARC
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| 520 | |a A method for the full determination of the third-order nonlinear coherent anti-Stokes Raman scattering (CARS) susceptibility is presented, which relies on phase control of a single ultrabroadband femtosecond laser pulse. A narrowband phase gate is scanned to perform double quadrature spectral interferometry, which reveals amplitude and phase of a multiplex CARS field. A single calibration measurement in a nonresonant sample allows for the characterization of the susceptibility in amplitude and phase. This scheme is demonstrated experimentally for the fingerprint region of toluene. | ||
| 650 | 4 | |a Coherent antistokes Raman scattering spectroscopy | |
| 650 | 4 | |a Heterodyne detection | |
| 650 | 4 | |a Nonlinear susceptibility | |
| 650 | 4 | |a Phase measurement | |
| 650 | 4 | |a Raman scattering | |
| 650 | 4 | |a Raman spectroscopy | |
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