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Direct signatures of light-induced conical intersections on the field-dressed spectrum of Na2

Rovibronic spectra of the field-dressed homonuclear diatomic Na2 molecule are investigated to identify direct signatures of the light-induced conical intersection (LICI) on the spectrum. The theoretical framework formulated allows the computation of the (1) field-dressed rovibronic states induced by...

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Main Authors: Szidarovszky, Tamás (Author) , Cederbaum, Lorenz S. (Author)
Format: Article (Journal)
Language:English
Published: May 7, 2018
In: The journal of physical chemistry letters
Year: 2018, Volume: 9, Issue: 11, Pages: 2739-2745
ISSN:1948-7185
DOI:10.1021/acs.jpclett.8b01102
Online Access:Verlag, Volltext: https://doi.org/10.1021/acs.jpclett.8b01102
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Author Notes:Tamás Szidarovszky, Gábor J. Halász, Attila G. Császár, Lorenz S. Cederbaum, Ágnes Vibók

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520 |a Rovibronic spectra of the field-dressed homonuclear diatomic Na2 molecule are investigated to identify direct signatures of the light-induced conical intersection (LICI) on the spectrum. The theoretical framework formulated allows the computation of the (1) field-dressed rovibronic states induced by a medium-intensity continuous-wave laser light and the (2) transition amplitudes between these field-dressed states with respect to an additional weak probe pulse. The field-dressed spectrum features absorption peaks resembling the field-free spectrum as well as stimulated emission peaks corresponding to transitions not visible in the field-free case. By investigating the dependence of the field-dressed spectra on the dressing-field wavelength, in both full- and reduced-dimensional simulations, direct signatures of the LICI can be identified. These signatures include (1) the appearance of new peaks and the splitting of peaks for both absorption and stimulated emission and (2) the manifestation of an intensity-borrowing effect in the field-dressed spectrum. 
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