How adsorbates alter the metallic behavior of quasi-1D electron systems of the Si(5\hspace0.167em5\hspace0.167em3)-Au surface
The plasmonic signals of quasi-1D electron systems are a clear and direct measure of their metallic behavior. Due to the finite size of such systems in reality, plasmonic signals from a gold-induced superstructure on Si(5 5 3) can be studied with infrared spectroscopy. The infrared spectroscopic fea...
Gespeichert in:
| Hauptverfasser: | , , , , , |
|---|---|
| Dokumenttyp: | Article (Journal) |
| Sprache: | Englisch |
| Veröffentlicht: |
11 March 2019
|
| In: |
Journal of physics. Condensed matter
Year: 2019, Jahrgang: 31, Heft: 19 |
| ISSN: | 1361-648X |
| DOI: | 10.1088/1361-648X/ab0710 |
| Online-Zugang: | Verlag, Volltext: https://doi.org/10.1088/1361-648X/ab0710 Verlag, Volltext: https://doi.org/10.1088%2F1361-648x%2Fab0710 
|
| Verfasserangaben: | Michael Tzschoppe, Christian Huck, Fabian Hötzel, Benjamin Günther, Zamin Mamiyev, Andrey Butkevich, Constantin Ulrich, Lutz H. Gade and Annemarie Pucci |
MARC
| LEADER | 00000caa a2200000 c 4500 | ||
|---|---|---|---|
| 001 | 1666223611 | ||
| 003 | DE-627 | ||
| 005 | 20230427154353.0 | ||
| 007 | cr uuu---uuuuu | ||
| 008 | 190523s2019 xx |||||o 00| ||eng c | ||
| 024 | 7 | |a 10.1088/1361-648X/ab0710 |2 doi | |
| 035 | |a (DE-627)1666223611 | ||
| 035 | |a (DE-599)KXP1666223611 | ||
| 035 | |a (OCoLC)1341225413 | ||
| 040 | |a DE-627 |b ger |c DE-627 |e rda | ||
| 041 | |a eng | ||
| 084 | |a 29 |2 sdnb | ||
| 100 | 1 | |a Tzschoppe, Michael |d 1991- |e VerfasserIn |0 (DE-588)1155250222 |0 (DE-627)1016567154 |0 (DE-576)501492577 |4 aut | |
| 245 | 1 | 0 | |a How adsorbates alter the metallic behavior of quasi-1D electron systems of the Si(5\hspace0.167em5\hspace0.167em3)-Au surface |c Michael Tzschoppe, Christian Huck, Fabian Hötzel, Benjamin Günther, Zamin Mamiyev, Andrey Butkevich, Constantin Ulrich, Lutz H. Gade and Annemarie Pucci |
| 264 | 1 | |c 11 March 2019 | |
| 300 | |a 9 | ||
| 336 | |a Text |b txt |2 rdacontent | ||
| 337 | |a Computermedien |b c |2 rdamedia | ||
| 338 | |a Online-Ressource |b cr |2 rdacarrier | ||
| 500 | |a Gesehen am 23.05.2019 | ||
| 520 | |a The plasmonic signals of quasi-1D electron systems are a clear and direct measure of their metallic behavior. Due to the finite size of such systems in reality, plasmonic signals from a gold-induced superstructure on Si(5 5 3) can be studied with infrared spectroscopy. The infrared spectroscopic features have turned out to be extremely sensitive to adsorbates. Even without geometrical changes of the surface superstructure, the effects of doping, of the adsorbate induced electronic surface scattering, and of the electronic polarizability changes on top of the substrate surface give rise to measurable changes of the plasmonic signal. Especially strong changes of the plasmonic signal have been observed for gold, oxygen, and hydrogen exposure. The plasmonic resonance gradually disappears under these exposures, indicating the transion to an insulating behavior, which is in accordance with published results obtained from other experimental methods. For C70 and, as shown here for the first time, TAPP-Br, the plasmonic signal almost retains its original intensity even up to coverages of many monolayers. For C70, the changes of the spectral shape, e.g. of electronic damping and of the resonance position, were also found to be marginal. On the other hand, TAPP-Br adsorption shifts the plasmonic resonance to higher frequencies and strongly increases the electronic damping. Given the dispersion relation for plasmonic resonances of 1D electron systems, the findings for TAPP-Br indicate a push-back effect and therefore stronger confinement of the free charge carriers in the quasi-one-dimensonal channel due to the coverage by the flat TAPP-Br molecules. On the gold-doped Si(5 5 3)-Au surface TAPP-Br acts as counter dopant and increases the plasmonic signal. | ||
| 700 | 1 | |a Huck, Christian |e VerfasserIn |0 (DE-588)1081576340 |0 (DE-627)846342065 |0 (DE-576)454553374 |4 aut | |
| 700 | 1 | |a Hötzel, Fabian |d 1988- |e VerfasserIn |0 (DE-588)1125659114 |0 (DE-627)880321741 |0 (DE-576)483537683 |4 aut | |
| 700 | 1 | |a Günther, Benjamin |d 1989- |e VerfasserIn |0 (DE-588)1148145656 |0 (DE-627)1008139734 |0 (DE-576)496186914 |4 aut | |
| 700 | 1 | |a Gade, Lutz H. |d 1963- |e VerfasserIn |0 (DE-588)1019812737 |0 (DE-627)691026750 |0 (DE-576)358881870 |4 aut | |
| 700 | 1 | |a Pucci, Annemarie |e VerfasserIn |0 (DE-588)1020648783 |0 (DE-627)691291969 |0 (DE-576)361698739 |4 aut | |
| 773 | 0 | 8 | |i Enthalten in |t Journal of physics. Condensed matter |d Bristol : IOP Publ., 1989 |g 31(2019,19) Artikel-Nummer 195001, 9 Seiten |h Online-Ressource |w (DE-627)268759936 |w (DE-600)1472968-4 |w (DE-576)07761013X |x 1361-648X |7 nnas |a How adsorbates alter the metallic behavior of quasi-1D electron systems of the Si(5\hspace0.167em5\hspace0.167em3)-Au surface |
| 773 | 1 | 8 | |g volume:31 |g year:2019 |g number:19 |g elocationid:195001 |g extent:9 |a How adsorbates alter the metallic behavior of quasi-1D electron systems of the Si(5\hspace0.167em5\hspace0.167em3)-Au surface |
| 856 | 4 | 0 | |u https://doi.org/10.1088/1361-648X/ab0710 |x Verlag |x Resolving-System |3 Volltext |
| 856 | 4 | 0 | |u https://doi.org/10.1088%2F1361-648x%2Fab0710 |x Verlag |3 Volltext |
| 951 | |a AR | ||
| 992 | |a 20190523 | ||
| 993 | |a Article | ||
| 994 | |a 2019 | ||
| 998 | |g 1020648783 |a Pucci, Annemarie |m 1020648783:Pucci, Annemarie |d 130000 |d 130700 |e 130000PP1020648783 |e 130700PP1020648783 |k 0/130000/ |k 1/130000/130700/ |p 9 |y j | ||
| 998 | |g 1019812737 |a Gade, Lutz H. |m 1019812737:Gade, Lutz H. |d 120000 |d 120200 |e 120000PG1019812737 |e 120200PG1019812737 |k 0/120000/ |k 1/120000/120200/ |p 8 | ||
| 998 | |g 1148145656 |a Günther, Benjamin |m 1148145656:Günther, Benjamin |d 500000 |d 501249 |e 500000PG1148145656 |e 501249PG1148145656 |k 0/500000/ |k 1/500000/501249/ |p 4 | ||
| 998 | |g 1125659114 |a Hötzel, Fabian |m 1125659114:Hötzel, Fabian |p 3 | ||
| 998 | |g 1081576340 |a Huck, Christian |m 1081576340:Huck, Christian |d 130000 |d 130700 |e 130000PH1081576340 |e 130700PH1081576340 |k 0/130000/ |k 1/130000/130700/ |p 2 | ||
| 998 | |g 1155250222 |a Tzschoppe, Michael |m 1155250222:Tzschoppe, Michael |d 130000 |d 130700 |e 130000PT1155250222 |e 130700PT1155250222 |k 0/130000/ |k 1/130000/130700/ |p 1 |x j | ||
| 999 | |a KXP-PPN1666223611 |e 3479084265 | ||
| BIB | |a Y | ||
| SER | |a journal | ||
| JSO | |a {"language":["eng"],"name":{"displayForm":["Michael Tzschoppe, Christian Huck, Fabian Hötzel, Benjamin Günther, Zamin Mamiyev, Andrey Butkevich, Constantin Ulrich, Lutz H. Gade and Annemarie Pucci"]},"type":{"bibl":"article-journal","media":"Online-Ressource"},"person":[{"display":"Tzschoppe, Michael","given":"Michael","role":"aut","family":"Tzschoppe"},{"role":"aut","given":"Christian","display":"Huck, Christian","family":"Huck"},{"given":"Fabian","display":"Hötzel, Fabian","role":"aut","family":"Hötzel"},{"family":"Günther","role":"aut","display":"Günther, Benjamin","given":"Benjamin"},{"family":"Gade","role":"aut","display":"Gade, Lutz H.","given":"Lutz H."},{"given":"Annemarie","display":"Pucci, Annemarie","role":"aut","family":"Pucci"}],"title":[{"title_sort":"How adsorbates alter the metallic behavior of quasi-1D electron systems of the Si(5\\hspace0.167em5\\hspace0.167em3)-Au surface","title":"How adsorbates alter the metallic behavior of quasi-1D electron systems of the Si(5\\hspace0.167em5\\hspace0.167em3)-Au surface"}],"physDesc":[{"extent":"9 S."}],"id":{"doi":["10.1088/1361-648X/ab0710"],"eki":["1666223611"]},"origin":[{"dateIssuedDisp":"11 March 2019","dateIssuedKey":"2019"}],"note":["Gesehen am 23.05.2019"],"recId":"1666223611","relHost":[{"id":{"issn":["1361-648X"],"doi":["10.1088/issn.0953-8984"],"zdb":["1472968-4"],"eki":["268759936"]},"language":["eng"],"recId":"268759936","note":["Gesehen am 11.04.2022"],"origin":[{"dateIssuedKey":"1989","publisher":"IOP Publ.","dateIssuedDisp":"1989-","publisherPlace":"Bristol"}],"pubHistory":["1.1989 -"],"title":[{"title":"Journal of physics","title_sort":"Journal of physics","partname":"Condensed matter"}],"part":{"text":"31(2019,19) Artikel-Nummer 195001, 9 Seiten","year":"2019","issue":"19","extent":"9","volume":"31"},"physDesc":[{"extent":"Online-Ressource"}],"disp":"How adsorbates alter the metallic behavior of quasi-1D electron systems of the Si(5\\hspace0.167em5\\hspace0.167em3)-Au surfaceJournal of physics. Condensed matter","type":{"media":"Online-Ressource","bibl":"periodical"},"titleAlt":[{"title":"Journal of physics / Condensed matter"}]}]} | ||
| SRT | |a TZSCHOPPEMHOWADSORBA1120 | ||