Site-selective probe of magnetic excitations in rare-earth nickelates using resonant inelastic X-ray scattering

We use high-resolution resonant inelastic x-ray scattering (RIXS) to study a thin film of NdNiO3, a compound whose unusual spin- and bond-ordered electronic ground state has been of long-standing interest. Below the magnetic ordering temperature, we observe well-defined collective magnon excitations...

Ausführliche Beschreibung

Gespeichert in:
Bibliographische Detailangaben
Hauptverfasser: Lu, Yi (VerfasserIn) , Haverkort, Maurits W. (VerfasserIn)
Dokumenttyp: Article (Journal)
Sprache:Englisch
Veröffentlicht: 18 July 2018
In: Physical review. X, Expanding access
Year: 2018, Jahrgang: 8, Heft: 3
ISSN:2160-3308
DOI:10.1103/PhysRevX.8.031014
Online-Zugang:Verlag, Volltext: https://doi.org/10.1103/PhysRevX.8.031014
Verlag, Volltext: https://link.aps.org/doi/10.1103/PhysRevX.8.031014
Volltext
Verfasserangaben:Y. Lu, D. Betto, K. Fürsich, H. Suzuki, H.-H. Kim, G. Cristiani, G. Logvenov, N. B. Brookes, E. Benckiser, M. W. Haverkort, G. Khaliullin, M. Le Tacon, M. Minola, and B. Keimer

MARC

LEADER 00000caa a2200000 c 4500
001 1669423727
003 DE-627
005 20220816193726.0
007 cr uuu---uuuuu
008 190718s2018 xx |||||o 00| ||eng c
024 7 |a 10.1103/PhysRevX.8.031014  |2 doi 
035 |a (DE-627)1669423727 
035 |a (DE-599)KXP1669423727 
035 |a (OCoLC)1341233983 
040 |a DE-627  |b ger  |c DE-627  |e rda 
041 |a eng 
084 |a 29  |2 sdnb 
100 1 |a Lu, Yi  |e VerfasserIn  |0 (DE-588)1140136585  |0 (DE-627)898252679  |0 (DE-576)49366713X  |4 aut 
245 1 0 |a Site-selective probe of magnetic excitations in rare-earth nickelates using resonant inelastic X-ray scattering  |c Y. Lu, D. Betto, K. Fürsich, H. Suzuki, H.-H. Kim, G. Cristiani, G. Logvenov, N. B. Brookes, E. Benckiser, M. W. Haverkort, G. Khaliullin, M. Le Tacon, M. Minola, and B. Keimer 
264 1 |c 18 July 2018 
300 |b Diagramme 
300 |a 9 
336 |a Text  |b txt  |2 rdacontent 
337 |a Computermedien  |b c  |2 rdamedia 
338 |a Online-Ressource  |b cr  |2 rdacarrier 
500 |a Gesehen am 18.07.2019 
520 |a We use high-resolution resonant inelastic x-ray scattering (RIXS) to study a thin film of NdNiO3, a compound whose unusual spin- and bond-ordered electronic ground state has been of long-standing interest. Below the magnetic ordering temperature, we observe well-defined collective magnon excitations along different high-symmetry directions in momentum space. The magnetic spectra depend strongly on the incident photon energy, which we attribute to RIXS coupling to different local electronic configurations of the expanded and compressed NiO6 octahedra in the bond-ordered state. Both the noncollinear magnetic ground state and the observed site-dependent magnon excitations are well described by a model that assumes strong competition between the antiferromagnetic superexchange and ferromagnetic double-exchange interactions. Our study provides direct insight into the magnetic dynamics and exchange interactions of the rare-earth nickelates and demonstrates that RIXS can serve as a site-selective probe of magnetism in these and other materials. 
700 1 |a Haverkort, Maurits W.  |d 1976-  |e VerfasserIn  |0 (DE-588)130132047  |0 (DE-627)491717946  |0 (DE-576)257824006  |4 aut 
773 0 8 |i Enthalten in  |t Physical review. X, Expanding access  |d College Park, Md. : APS, 2011  |g 8 (2018,3) Artikel-Nummer 031014, Seite 1-9, 9 Seiten  |h Online-Ressource  |w (DE-627)666214115  |w (DE-600)2622565-7  |w (DE-576)348749260  |x 2160-3308  |7 nnas  |a Site-selective probe of magnetic excitations in rare-earth nickelates using resonant inelastic X-ray scattering 
773 1 8 |g volume:8  |g year:2018  |g number:3  |g extent:9  |a Site-selective probe of magnetic excitations in rare-earth nickelates using resonant inelastic X-ray scattering 
856 4 0 |u https://doi.org/10.1103/PhysRevX.8.031014  |x Verlag  |x Resolving-System  |3 Volltext 
856 4 0 |u https://link.aps.org/doi/10.1103/PhysRevX.8.031014  |x Verlag  |3 Volltext 
951 |a AR 
992 |a 20190718 
993 |a Article 
994 |a 2018 
998 |g 1140136585  |a Lu, Yi  |m 1140136585:Lu, Yi  |d 130000  |d 130300  |e 130000PL1140136585  |e 130300PL1140136585  |k 0/130000/  |k 1/130000/130300/  |p 1  |x j 
998 |g 130132047  |a Haverkort, Maurits W.  |m 130132047:Haverkort, Maurits W.  |d 130000  |d 130300  |e 130000PH130132047  |e 130300PH130132047  |k 0/130000/  |k 1/130000/130300/  |p 10 
999 |a KXP-PPN1669423727  |e 3494770972 
BIB |a Y 
SER |a journal 
JSO |a {"recId":"1669423727","note":["Gesehen am 18.07.2019"],"name":{"displayForm":["Y. Lu, D. Betto, K. Fürsich, H. Suzuki, H.-H. Kim, G. Cristiani, G. Logvenov, N. B. Brookes, E. Benckiser, M. W. Haverkort, G. Khaliullin, M. Le Tacon, M. Minola, and B. Keimer"]},"relHost":[{"part":{"extent":"9","year":"2018","volume":"8","text":"8 (2018,3) Artikel-Nummer 031014, Seite 1-9, 9 Seiten","issue":"3"},"physDesc":[{"extent":"Online-Ressource"}],"title":[{"title_sort":"Physical review","title":"Physical review","partname":"Expanding access"}],"titleAlt":[{"title":"Physical review / X"},{"title":"PRX"}],"origin":[{"publisher":"APS","dateIssuedKey":"2011","dateIssuedDisp":"2011-","publisherPlace":"College Park, Md."}],"recId":"666214115","pubHistory":["1.2011 -"],"note":["Gesehen am 05.11.25"],"name":{"displayForm":["The American Physical Society"]},"disp":"Site-selective probe of magnetic excitations in rare-earth nickelates using resonant inelastic X-ray scatteringPhysical review. X, Expanding access","id":{"eki":["666214115"],"zdb":["2622565-7"],"issn":["2160-3308"]},"type":{"bibl":"periodical","media":"Online-Ressource"},"language":["eng"],"corporate":[{"display":"American Physical Society","role":"isb"}]}],"person":[{"role":"aut","given":"Yi","display":"Lu, Yi","family":"Lu"},{"role":"aut","display":"Haverkort, Maurits W.","family":"Haverkort","given":"Maurits W."}],"physDesc":[{"noteIll":"Diagramme","extent":"9 S."}],"title":[{"title":"Site-selective probe of magnetic excitations in rare-earth nickelates using resonant inelastic X-ray scattering","title_sort":"Site-selective probe of magnetic excitations in rare-earth nickelates using resonant inelastic X-ray scattering"}],"id":{"doi":["10.1103/PhysRevX.8.031014"],"eki":["1669423727"]},"language":["eng"],"type":{"media":"Online-Ressource","bibl":"article-journal"},"origin":[{"dateIssuedDisp":"18 July 2018","dateIssuedKey":"2018"}]} 
SRT |a LUYIHAVERKSITESELECT1820