Direct evidence for radiative charge transfer after inner-shell excitation and ionization of large clusters
We directly observe radiative charge transfer (RCT) in Ne clusters by dispersed vacuum-ultraviolet photon detection. The doubly ionized Ne2+- initial states of RCT are populated after resonant 1s-3p photoexcitation or 1s photoionization of Ne n clusters with . These states relax further producing Ne...
Saved in:
| Main Authors: | , |
|---|---|
| Format: | Article (Journal) |
| Language: | English |
| Published: |
16 January 2018
|
| In: |
New journal of physics
Year: 2018, Volume: 20, Issue: 1 |
| ISSN: | 1367-2630 |
| DOI: | 10.1088/1367-2630/aaa4af |
| Online Access: | Verlag, Volltext: https://doi.org/10.1088/1367-2630/aaa4af Verlag, Volltext: https://doi.org/10.1088%2F1367-2630%2Faaa4af 
|
| Author Notes: | Andreas Hans, Vasili Stumpf, Xaver Holzapfel, Florian Wiegandt, Philipp Schmidt, Christian Ozga, Philipp Reiß, Ltaief Ben Ltaief, Catmarna Kästner-Wetekam, Till Jahnke, Arno Ehresmann, Philipp V. Demekhin, Kirill Gokhberg, and Andre Knie |
MARC
| LEADER | 00000caa a2200000 c 4500 | ||
|---|---|---|---|
| 001 | 1672099005 | ||
| 003 | DE-627 | ||
| 005 | 20230426085855.0 | ||
| 007 | cr uuu---uuuuu | ||
| 008 | 190826s2018 xx |||||o 00| ||eng c | ||
| 024 | 7 | |a 10.1088/1367-2630/aaa4af |2 doi | |
| 035 | |a (DE-627)1672099005 | ||
| 035 | |a (DE-599)KXP1672099005 | ||
| 035 | |a (OCoLC)1341238285 | ||
| 040 | |a DE-627 |b ger |c DE-627 |e rda | ||
| 041 | |a eng | ||
| 084 | |a 30 |2 sdnb | ||
| 100 | 1 | |a Hans, Andreas |e VerfasserIn |0 (DE-588)1193433215 |0 (DE-627)1672098882 |4 aut | |
| 245 | 1 | 0 | |a Direct evidence for radiative charge transfer after inner-shell excitation and ionization of large clusters |c Andreas Hans, Vasili Stumpf, Xaver Holzapfel, Florian Wiegandt, Philipp Schmidt, Christian Ozga, Philipp Reiß, Ltaief Ben Ltaief, Catmarna Kästner-Wetekam, Till Jahnke, Arno Ehresmann, Philipp V. Demekhin, Kirill Gokhberg, and Andre Knie |
| 264 | 1 | |c 16 January 2018 | |
| 300 | |a 7 | ||
| 336 | |a Text |b txt |2 rdacontent | ||
| 337 | |a Computermedien |b c |2 rdamedia | ||
| 338 | |a Online-Ressource |b cr |2 rdacarrier | ||
| 500 | |a Gesehen am 26.08.2019 | ||
| 520 | |a We directly observe radiative charge transfer (RCT) in Ne clusters by dispersed vacuum-ultraviolet photon detection. The doubly ionized Ne2+- initial states of RCT are populated after resonant 1s-3p photoexcitation or 1s photoionization of Ne n clusters with . These states relax further producing Ne+-Ne+- final states, and the RCT photon is emitted. Ab initio calculations assign the observed RCT signal to the initial state, while transitions from other possible initial states are proposed to be quenched by competing relaxation processes. The present results are in agreement with the commonly discussed scenario, where the doubly ionized atom in a noble gas cluster forms a dimer which dissipates its vibrational energy on a picosecond timescale. Our study complements the picture of the RCT process in weakly bound clusters, providing information which is inaccessible by charged particle detection techniques. | ||
| 700 | 1 | |a Stumpf, Vasili |e VerfasserIn |0 (DE-588)112461107X |0 (DE-627)878837329 |0 (DE-576)483055565 |4 aut | |
| 773 | 0 | 8 | |i Enthalten in |t New journal of physics |d [Bad Honnef] : Dt. Physikalische Ges., 1999 |g 20(2018,1) Artikel-Nummer 012001, 7 Seiten |h Online-Ressource |w (DE-627)265510562 |w (DE-600)1464444-7 |w (DE-576)078991846 |x 1367-2630 |7 nnas |a Direct evidence for radiative charge transfer after inner-shell excitation and ionization of large clusters |
| 773 | 1 | 8 | |g volume:20 |g year:2018 |g number:1 |g extent:7 |a Direct evidence for radiative charge transfer after inner-shell excitation and ionization of large clusters |
| 856 | 4 | 0 | |u https://doi.org/10.1088/1367-2630/aaa4af |x Verlag |x Resolving-System |3 Volltext |
| 856 | 4 | 0 | |u https://doi.org/10.1088%2F1367-2630%2Faaa4af |x Verlag |3 Volltext |
| 951 | |a AR | ||
| 992 | |a 20190826 | ||
| 993 | |a Article | ||
| 994 | |a 2018 | ||
| 998 | |g 112461107X |a Stumpf, Vasili |m 112461107X:Stumpf, Vasili |d 120000 |d 120300 |e 120000PS112461107X |e 120300PS112461107X |k 0/120000/ |k 1/120000/120300/ |p 2 | ||
| 999 | |a KXP-PPN1672099005 |e 3508845907 | ||
| BIB | |a Y | ||
| SER | |a journal | ||
| JSO | |a {"language":["eng"],"recId":"1672099005","type":{"bibl":"article-journal","media":"Online-Ressource"},"note":["Gesehen am 26.08.2019"],"title":[{"title":"Direct evidence for radiative charge transfer after inner-shell excitation and ionization of large clusters","title_sort":"Direct evidence for radiative charge transfer after inner-shell excitation and ionization of large clusters"}],"person":[{"family":"Hans","given":"Andreas","display":"Hans, Andreas","roleDisplay":"VerfasserIn","role":"aut"},{"family":"Stumpf","given":"Vasili","roleDisplay":"VerfasserIn","display":"Stumpf, Vasili","role":"aut"}],"relHost":[{"id":{"issn":["1367-2630"],"zdb":["1464444-7"],"eki":["265510562"]},"origin":[{"publisherPlace":"[Bad Honnef] ; [London]","dateIssuedKey":"1999","publisher":"Dt. Physikalische Ges. ; IOP","dateIssuedDisp":"1999-"}],"name":{"displayForm":["Deutsche Physikalische Gesellschaft ; IOP, Institute of Physics"]},"physDesc":[{"extent":"Online-Ressource"}],"title":[{"title":"New journal of physics","subtitle":"the open-access journal for physics","title_sort":"New journal of physics"}],"part":{"issue":"1","year":"2018","extent":"7","text":"20(2018,1) Artikel-Nummer 012001, 7 Seiten","volume":"20"},"pubHistory":["1.1998/99(1999) -"],"corporate":[{"role":"isb","roleDisplay":"Herausgebendes Organ","display":"Institute of Physics"},{"role":"isb","display":"Deutsche Physikalische Gesellschaft","roleDisplay":"Herausgebendes Organ"}],"language":["eng"],"recId":"265510562","disp":"Direct evidence for radiative charge transfer after inner-shell excitation and ionization of large clustersNew journal of physics","note":["Gesehen am 16.06.20"],"type":{"bibl":"periodical","media":"Online-Ressource"}}],"physDesc":[{"extent":"7 S."}],"id":{"doi":["10.1088/1367-2630/aaa4af"],"eki":["1672099005"]},"origin":[{"dateIssuedDisp":"16 January 2018","dateIssuedKey":"2018"}],"name":{"displayForm":["Andreas Hans, Vasili Stumpf, Xaver Holzapfel, Florian Wiegandt, Philipp Schmidt, Christian Ozga, Philipp Reiß, Ltaief Ben Ltaief, Catmarna Kästner-Wetekam, Till Jahnke, Arno Ehresmann, Philipp V. Demekhin, Kirill Gokhberg, and Andre Knie"]}} | ||
| SRT | |a HANSANDREADIRECTEVID1620 | ||