A fast and sensitive method for the continuous in situ determination of dissolved methane and its [delta]13C-isotope ratio in surface waters
A fast and sensitive method for the continuous determination of methane (CH4) and its stable carbon isotopic values (δ13C-CH4) in surface waters was developed by applying a vacuum to a gas/liquid exchange membrane and measuring the extracted gases by a portable cavity ring-down spectroscopy analyser...
Gespeichert in:
| Hauptverfasser: | , , , , |
|---|---|
| Dokumenttyp: | Article (Journal) |
| Sprache: | Englisch |
| Veröffentlicht: |
27 April 2018
|
| In: |
Limnology and oceanography. Methods
Year: 2018, Jahrgang: 16, Heft: 5, Pages: 273-285 |
| ISSN: | 1541-5856 |
| DOI: | 10.1002/lom3.10244 |
| Online-Zugang: | Verlag, Volltext: https://doi.org/10.1002/lom3.10244 Verlag, Volltext: https://aslopubs.onlinelibrary.wiley.com/doi/abs/10.1002/lom3.10244 
|
| Verfasserangaben: | Jan F. Hartmann, Torben Gentz, Amanda Schiller, Markus Greule, Hans-Peter Grossart, Danny Ionescu, Frank Keppler, Karla Martinez‐Cruz, Armando Sepulveda‐Jauregui, Margot Isenbeck‐Schröter |
MARC
| LEADER | 00000caa a2200000 c 4500 | ||
|---|---|---|---|
| 001 | 1675991774 | ||
| 003 | DE-627 | ||
| 005 | 20220816221235.0 | ||
| 007 | cr uuu---uuuuu | ||
| 008 | 190905s2018 xx |||||o 00| ||eng c | ||
| 024 | 7 | |a 10.1002/lom3.10244 |2 doi | |
| 035 | |a (DE-627)1675991774 | ||
| 035 | |a (DE-599)KXP1675991774 | ||
| 035 | |a (OCoLC)1341242533 | ||
| 040 | |a DE-627 |b ger |c DE-627 |e rda | ||
| 041 | |a eng | ||
| 084 | |a 31 |2 sdnb | ||
| 100 | 1 | |a Kleint, Jan F. |e VerfasserIn |0 (DE-588)1055834907 |0 (DE-627)792720393 |0 (DE-576)41189224X |4 aut | |
| 245 | 1 | 2 | |a A fast and sensitive method for the continuous in situ determination of dissolved methane and its [delta]13C-isotope ratio in surface waters |c Jan F. Hartmann, Torben Gentz, Amanda Schiller, Markus Greule, Hans-Peter Grossart, Danny Ionescu, Frank Keppler, Karla Martinez‐Cruz, Armando Sepulveda‐Jauregui, Margot Isenbeck‐Schröter |
| 264 | 1 | |c 27 April 2018 | |
| 300 | |a 13 | ||
| 336 | |a Text |b txt |2 rdacontent | ||
| 337 | |a Computermedien |b c |2 rdamedia | ||
| 338 | |a Online-Ressource |b cr |2 rdacarrier | ||
| 500 | |a Im Titel ist "delta" als griechischer Buchstabe dargestellt | ||
| 500 | |a im Titel ist die Zahl "13" hochgestellt | ||
| 500 | |a Gesehen am 05.09.2019 | ||
| 520 | |a A fast and sensitive method for the continuous determination of methane (CH4) and its stable carbon isotopic values (δ13C-CH4) in surface waters was developed by applying a vacuum to a gas/liquid exchange membrane and measuring the extracted gases by a portable cavity ring-down spectroscopy analyser (M-CRDS). The M-CRDS was calibrated and characterized for CH4 concentration and δ13C-CH4 with synthetic water standards. The detection limit of the M-CRDS for the simultaneous determination of CH4 and δ13C-CH4 is 3.6 nmol L−1 CH4. A measurement precision of CH4 concentrations and δ13C-CH4 in the range of 1.1%, respectively, 1.7‰ (1σ) and accuracy (1.3%, respectively, 0.8‰ [1σ]) was achieved for single measurements and averaging times of 10 min. The response time τ of 57 ± 5 s allow determination of δ13C-CH4 values more than twice as fast than other methods. The demonstrated M-CRDS method was applied and tested for Lake Stechlin (Germany) and compared with the headspace-gas chromatography and fast membrane CH4 concentration methods. Maximum CH4 concentrations (577 nmol L−1) and lightest δ13C-CH4 (−35.2‰) were found around the thermocline in depth profile measurements. The M-CRDS-method was in good agreement with other methods. Temporal variations in CH4 concentration and δ13C-CH4 obtained in 24 h measurements indicate either local methane production/oxidation or physical variations in the thermocline. Therefore, these results illustrate the need of fast and sensitive analyses to achieve a better understanding of different mechanisms and pathways of CH4 formation in aquatic environments. | ||
| 700 | 1 | |a Schiller, Amanda |e VerfasserIn |0 (DE-588)1081902264 |0 (DE-627)846776170 |0 (DE-576)45485286X |4 aut | |
| 700 | 1 | |a Greule, Markus |d 1977- |e VerfasserIn |0 (DE-588)134158555 |0 (DE-627)56210626X |0 (DE-576)300347944 |4 aut | |
| 700 | 1 | |a Keppler, Frank |d 1967- |e VerfasserIn |0 (DE-588)122072537 |0 (DE-627)705762130 |0 (DE-576)293077991 |4 aut | |
| 700 | 1 | |a Isenbeck-Schröter, Margot |e VerfasserIn |0 (DE-588)1019894997 |0 (DE-627)691048991 |0 (DE-576)359058973 |4 aut | |
| 773 | 0 | 8 | |i Enthalten in |t Limnology and oceanography. Methods |d Oxford [u.a.] : Wiley-Blackwell, 2003 |g 16(2018), 5, Seite 273-285 |h Online-Ressource |w (DE-627)395967511 |w (DE-600)2161715-6 |w (DE-576)261570625 |x 1541-5856 |7 nnas |a A fast and sensitive method for the continuous in situ determination of dissolved methane and its [delta]13C-isotope ratio in surface waters |
| 773 | 1 | 8 | |g volume:16 |g year:2018 |g number:5 |g pages:273-285 |g extent:13 |a A fast and sensitive method for the continuous in situ determination of dissolved methane and its [delta]13C-isotope ratio in surface waters |
| 856 | 4 | 0 | |u https://doi.org/10.1002/lom3.10244 |x Verlag |x Resolving-System |3 Volltext |
| 856 | 4 | 0 | |u https://aslopubs.onlinelibrary.wiley.com/doi/abs/10.1002/lom3.10244 |x Verlag |x Resolving-System |3 Volltext |
| 951 | |a AR | ||
| 992 | |a 20190905 | ||
| 993 | |a Article | ||
| 994 | |a 2018 | ||
| 998 | |g 1019894997 |a Isenbeck-Schröter, Margot |m 1019894997:Isenbeck-Schröter, Margot |d 120000 |d 121000 |e 120000PI1019894997 |e 121000PI1019894997 |k 0/120000/ |k 1/120000/121000/ |p 10 |y j | ||
| 998 | |g 122072537 |a Keppler, Frank |m 122072537:Keppler, Frank |d 120000 |d 121000 |d 700000 |d 729400 |e 120000PK122072537 |e 121000PK122072537 |e 700000PK122072537 |e 729400PK122072537 |k 0/120000/ |k 1/120000/121000/ |k 0/700000/ |k 1/700000/729400/ |p 7 | ||
| 998 | |g 134158555 |a Greule, Markus |m 134158555:Greule, Markus |d 120000 |d 121000 |e 120000PG134158555 |e 121000PG134158555 |k 0/120000/ |k 1/120000/121000/ |p 4 | ||
| 998 | |g 1081902264 |a Schiller, Amanda |m 1081902264:Schiller, Amanda |p 3 | ||
| 998 | |g 1055834907 |a Kleint, Jan F. |m 1055834907:Kleint, Jan F. |d 120000 |d 121000 |e 120000PK1055834907 |e 121000PK1055834907 |k 0/120000/ |k 1/120000/121000/ |p 1 |x j | ||
| 999 | |a KXP-PPN1675991774 |e 3511965578 | ||
| BIB | |a Y | ||
| SER | |a journal | ||
| JSO | |a {"name":{"displayForm":["Jan F. Hartmann, Torben Gentz, Amanda Schiller, Markus Greule, Hans-Peter Grossart, Danny Ionescu, Frank Keppler, Karla Martinez‐Cruz, Armando Sepulveda‐Jauregui, Margot Isenbeck‐Schröter"]},"physDesc":[{"extent":"13 S."}],"relHost":[{"note":["Gesehen am 14.03.25","Beteil. Körp. anfangs: American Society of Limnology and Oceanography"],"pubHistory":["1.2003 -"],"type":{"media":"Online-Ressource","bibl":"periodical"},"origin":[{"dateIssuedDisp":"2003-","publisher":"Wiley-Blackwell ; ASLO","publisherPlace":"Oxford [u.a.] ; Waco, Tex.","dateIssuedKey":"2003"}],"physDesc":[{"extent":"Online-Ressource"}],"title":[{"title":"Limnology and oceanography","title_sort":"Limnology and oceanography","partname":"Methods"}],"part":{"text":"16(2018), 5, Seite 273-285","extent":"13","volume":"16","year":"2018","pages":"273-285","issue":"5"},"name":{"displayForm":["ASLO, Association for the Sciences of Limnology and Oceanography"]},"titleAlt":[{"title":"Limnology and oceanography / Methods"}],"recId":"395967511","disp":"A fast and sensitive method for the continuous in situ determination of dissolved methane and its [delta]13C-isotope ratio in surface watersLimnology and oceanography. Methods","language":["eng"],"id":{"doi":["10.1002/(ISSN)1541-5856"],"zdb":["2161715-6"],"issn":["1541-5856"],"eki":["395967511"]}}],"type":{"bibl":"article-journal","media":"Online-Ressource"},"note":["Im Titel ist \"delta\" als griechischer Buchstabe dargestellt","im Titel ist die Zahl \"13\" hochgestellt","Gesehen am 05.09.2019"],"origin":[{"dateIssuedDisp":"27 April 2018","dateIssuedKey":"2018"}],"title":[{"title_sort":"fast and sensitive method for the continuous in situ determination of dissolved methane and its [delta]13C-isotope ratio in surface waters","title":"A fast and sensitive method for the continuous in situ determination of dissolved methane and its [delta]13C-isotope ratio in surface waters"}],"language":["eng"],"id":{"doi":["10.1002/lom3.10244"],"eki":["1675991774"]},"recId":"1675991774","person":[{"given":"Jan F.","roleDisplay":"VerfasserIn","display":"Kleint, Jan F.","family":"Kleint","role":"aut"},{"role":"aut","family":"Schiller","display":"Schiller, Amanda","given":"Amanda","roleDisplay":"VerfasserIn"},{"display":"Greule, Markus","given":"Markus","roleDisplay":"VerfasserIn","role":"aut","family":"Greule"},{"display":"Keppler, Frank","roleDisplay":"VerfasserIn","given":"Frank","role":"aut","family":"Keppler"},{"display":"Isenbeck-Schröter, Margot","roleDisplay":"VerfasserIn","given":"Margot","role":"aut","family":"Isenbeck-Schröter"}]} | ||
| SRT | |a KLEINTJANFFASTANDSEN2720 | ||