Gold(III)-catalyzed formal [3 + 2] annulations of N-Acyl sulfilimines with Ynamides for the synthesis of 4-Aminooxazoles
A gold-catalyzed formal 1,3-dipolar [3 + 2] annulation using readily accessible N-acyl sulfilimines and ynamides is reported. This reaction includes the cleavage of a N-S bond and subsequent C-O bond formation. In total, 30 oxazole derivatives bearing diverse functionalities could be prepared in 43-...
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| Hauptverfasser: | , , , , , , , |
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| Dokumenttyp: | Article (Journal) |
| Sprache: | Englisch |
| Veröffentlicht: |
April 9, 2019
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| In: |
Organic letters
Year: 2019, Jahrgang: 21, Heft: 8, Pages: 2937-2940 |
| ISSN: | 1523-7052 |
| DOI: | 10.1021/acs.orglett.9b01011 |
| Online-Zugang: | Verlag, Pay-per-use, Volltext: https://doi.org/10.1021/acs.orglett.9b01011
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| Verfasserangaben: | Xianhai Tian, Lina Song, Chunyu Han, Cheng Zhang, Yufeng Wu, Matthias Rudolph, Frank Rominger, and A. Stephen K. Hashmi |
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| 520 | |a A gold-catalyzed formal 1,3-dipolar [3 + 2] annulation using readily accessible N-acyl sulfilimines and ynamides is reported. This reaction includes the cleavage of a N-S bond and subsequent C-O bond formation. In total, 30 oxazole derivatives bearing diverse functionalities could be prepared in 43-98% yield from the corresponding sulfilimines and ynamides. | ||
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