Synthesis, crystal structures and dye removal properties of a series of metal-organic frameworks based on N-heterocyclic carboxylic acid ligands
Six functional metal-organic frameworks build by 4,4'-(1H-1,2,4-triazol-1-yl)methylenebis (benzonic acid) (H2tmlb), namely: [Zn4(tmlb)4(H2O)]n (1), [Ni4(tmlb)4(H2O)]n (2), [Cu(tmlb)]n (3), [Co(tmlb)]n (4), [Pb(tmlb)(H2O)]n (5), {[Zn(tmlb)(H2tmlb)]H2O}n (6), have been successfully synthesized. T...
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| Hauptverfasser: | , , , , , |
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| Dokumenttyp: | Article (Journal) |
| Sprache: | Englisch |
| Veröffentlicht: |
13 March 2019
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| In: |
Microporous and mesoporous materials
Year: 2019, Jahrgang: 282, Pages: 82-90 |
| ISSN: | 1873-3093 |
| DOI: | 10.1016/j.micromeso.2019.03.014 |
| Online-Zugang: | Verlag, Volltext: https://doi.org/10.1016/j.micromeso.2019.03.014 Verlag, Volltext: http://www.sciencedirect.com/science/article/pii/S1387181119301507 
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| Verfasserangaben: | Zi-ao Zong, Chuan-bin Fan, Xia Zhang, Xiang-min Meng, Fan Jin, Yu-hua Fan |
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| 245 | 1 | 0 | |a Synthesis, crystal structures and dye removal properties of a series of metal-organic frameworks based on N-heterocyclic carboxylic acid ligands |c Zi-ao Zong, Chuan-bin Fan, Xia Zhang, Xiang-min Meng, Fan Jin, Yu-hua Fan |
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| 520 | |a Six functional metal-organic frameworks build by 4,4'-(1H-1,2,4-triazol-1-yl)methylenebis (benzonic acid) (H2tmlb), namely: [Zn4(tmlb)4(H2O)]n (1), [Ni4(tmlb)4(H2O)]n (2), [Cu(tmlb)]n (3), [Co(tmlb)]n (4), [Pb(tmlb)(H2O)]n (5), {[Zn(tmlb)(H2tmlb)]H2O}n (6), have been successfully synthesized. The X-ray diffraction analysis show that the complexes 1 and 2 exhibited a two interpenetrating (3, 6, 6)-connected framework with a Schläfli symbol of (4·62)2 (42·610·83) topology. The complexes 3 and 4 show a two interpenetrating (3, 6)-connected net with (611·84) (63)2 topology. The complex 5 shows a (3, 8)-connected network with a point symbol of (4·62)2 (42·615·78·8·92) topology. The complex 6 exists a 2-fold interpenetrating topology framework and the point symbol is (6·6·6). Moreover, the photocatalytic studies show that complexes 1-5 have highly photocatalytic ability to degrade methylene blue (MB). In addition, the complex 6 can efficiently adsorb Congo red through H-bonds and the adsorption kinetic have been discussed. | ||
| 650 | 4 | |a Dye adsorption | |
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