Magnetism and the phase diagram of MnSb2O6
Static and dynamic magnetic properties of P¯31m-phase MnSb2O6 have been studied by means of muon-spin relaxation (μSR), high-frequency electron-spin resonance (HF-ESR), specific heat, and magnetization studies in magnetic fields up to 25 T. The data imply onset of long-range antiferromagnetic order...
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| Main Authors: | , , , |
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| Format: | Article (Journal) |
| Language: | English |
| Published: |
15 June 2018
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| In: |
Physical review
Year: 2018, Volume: 97, Issue: 22 |
| ISSN: | 2469-9969 |
| DOI: | 10.1103/PhysRevB.97.224416 |
| Online Access: | Resolving-System, Volltext: https://doi.org/10.1103/PhysRevB.97.224416 Verlag: https://link.aps.org/doi/10.1103/PhysRevB.97.224416 
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| Author Notes: | C. Koo, J. Werner, M. Tzschoppe, M. Abdel-Hafiez, P.K. Biswas, R. Sarkar, H.-H. Klauss, G.V. Raganyan, E.A. Ovchenkov, A. Yu. Nikulin, A.N. Vasiliev, E.A. Zvereva, and R. Klingeler |
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| 520 | |a Static and dynamic magnetic properties of P¯31m-phase MnSb2O6 have been studied by means of muon-spin relaxation (μSR), high-frequency electron-spin resonance (HF-ESR), specific heat, and magnetization studies in magnetic fields up to 25 T. The data imply onset of long-range antiferromagnetic order at TN = 8 K and a spin-flop-like transition at BSF ≈ 0.7-1 T. Below TN, muon asymmetry exhibits well-defined oscillations indicating a narrow distribution of the local fields. A competing antiferromagnetic phase appearing below TN2 = 5.3 K is evidenced by a step in the magnetization and a slight kink of the relaxation rate. Above TN, both μSR and HF-ESR data suggest short-range spin order. HF-ESR data show that local magnetic fields persist up to at least 12TN≈100 K. Analysis of the antiferromagnetic resonance modes and the thermodynamic spin-flop field suggest zero-field splitting of Δ≈18 GHz which implies small but finite magnetic anisotropy. | ||
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