Experimental evidence for ultrafast intermolecular relaxation processes in hydrated biomolecules

The authors study intermolecular Coulomb decay that occurs in a sample of THF and water in a reaction microscope employing triple-coincidence measurements of two ions and one electron. They find that ICD is a previously unconsidered effect between water and other organic molecules that are hydrogen-...

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Hauptverfasser: Ren, Xueguang (VerfasserIn) , Gokhberg, Kirill (VerfasserIn) , Dorn, Alexander (VerfasserIn)
Dokumenttyp: Article (Journal)
Sprache:Englisch
Veröffentlicht: 23 July 2018
In: Nature physics
Year: 2018, Jahrgang: 14, Heft: 10, Pages: 1062-1066
ISSN:1745-2481
DOI:10.1038/s41567-018-0214-9
Online-Zugang:Verlag, Volltext: https://doi.org/10.1038/s41567-018-0214-9
Verlag: https://www.nature.com/articles/s41567-018-0214-9
Volltext
Verfasserangaben:Xueguang Ren, Enliang Wang, Anna D. Skitnevskaya, Alexander B. Trofimov, Kirill Gokhberg and Alexander Dorn
Beschreibung
Zusammenfassung:The authors study intermolecular Coulomb decay that occurs in a sample of THF and water in a reaction microscope employing triple-coincidence measurements of two ions and one electron. They find that ICD is a previously unconsidered effect between water and other organic molecules that are hydrogen-bonded, with ICD outpacing proton transfer.
Beschreibung:Gesehen am 04.02.2020
Beschreibung:Online Resource
ISSN:1745-2481
DOI:10.1038/s41567-018-0214-9