Structure-property relationship of phenylene-based self-assembled monolayers for record low work function of indium tin oxide
Studying the structure-property relations of tailored dipolar phenyl and biphenylphosphonic acids, we report self-assembled monolayers with a significant decrease in the work function (WF) of indium-tin oxide (ITO) electrodes. Whereas the strengths of the dipoles are varied through the different mol...
Gespeichert in:
| Hauptverfasser: | , , , , , , , |
|---|---|
| Dokumenttyp: | Article (Journal) |
| Sprache: | Englisch |
| Veröffentlicht: |
20 June 2018
|
| In: |
The journal of physical chemistry letters
Year: 2018, Jahrgang: 9, Heft: 13, Pages: 3731-3737 |
| ISSN: | 1948-7185 |
| DOI: | 10.1021/acs.jpclett.8b01242 |
| Online-Zugang: | Verlag, lizenzpflichtig, Volltext: https://doi.org/10.1021/acs.jpclett.8b01242
|
| Verfasserangaben: | Frank S. Benneckendorf, Sabina Hillebrandt, Florian Ullrich, Valentina Rohnacher, Sebastian Hietzschold, Daniel Jänsch, Jan Freudenberg, Sebastian Beck, Eric Mankel, Wolfram Jaegermann, Annemarie Pucci, Uwe H.F. Bunz, and Klaus Müllen |
MARC
| LEADER | 00000caa a2200000 c 4500 | ||
|---|---|---|---|
| 001 | 1692260901 | ||
| 003 | DE-627 | ||
| 005 | 20220818011836.0 | ||
| 007 | cr uuu---uuuuu | ||
| 008 | 200311s2018 xx |||||o 00| ||eng c | ||
| 024 | 7 | |a 10.1021/acs.jpclett.8b01242 |2 doi | |
| 035 | |a (DE-627)1692260901 | ||
| 035 | |a (DE-599)KXP1692260901 | ||
| 035 | |a (OCoLC)1341310113 | ||
| 040 | |a DE-627 |b ger |c DE-627 |e rda | ||
| 041 | |a eng | ||
| 084 | |a 29 |2 sdnb | ||
| 100 | 1 | |a Benneckendorf, Frank S. |e VerfasserIn |0 (DE-588)1194346294 |0 (DE-627)167633131X |4 aut | |
| 245 | 1 | 0 | |a Structure-property relationship of phenylene-based self-assembled monolayers for record low work function of indium tin oxide |c Frank S. Benneckendorf, Sabina Hillebrandt, Florian Ullrich, Valentina Rohnacher, Sebastian Hietzschold, Daniel Jänsch, Jan Freudenberg, Sebastian Beck, Eric Mankel, Wolfram Jaegermann, Annemarie Pucci, Uwe H.F. Bunz, and Klaus Müllen |
| 264 | 1 | |c 20 June 2018 | |
| 300 | |a 7 | ||
| 336 | |a Text |b txt |2 rdacontent | ||
| 337 | |a Computermedien |b c |2 rdamedia | ||
| 338 | |a Online-Ressource |b cr |2 rdacarrier | ||
| 500 | |a Gesehen am 11.03.2020 | ||
| 520 | |a Studying the structure-property relations of tailored dipolar phenyl and biphenylphosphonic acids, we report self-assembled monolayers with a significant decrease in the work function (WF) of indium-tin oxide (ITO) electrodes. Whereas the strengths of the dipoles are varied through the different molecular lengths and the introduction of electron-withdrawing fluorine atoms, the surface energy is kept constant through the electron-donating N,N-dimethylamine head groups. The self-assembled monolayer formation and its modification of the electrodes are investigated via infrared reflection absorption spectroscopy, contact angle measurements, and photoelectron spectroscopy. The WF decrease in ITO correlates with increasing molecular dipoles. The lowest ever recorded WF of 3.7 eV is achieved with the fluorinated biphenylphosphonic acid. | ||
| 700 | 1 | |a Hillebrandt, Sabina |d 1987- |e VerfasserIn |0 (DE-588)107115737X |0 (DE-627)825616832 |0 (DE-576)432976299 |4 aut | |
| 700 | 1 | |a Rohnacher, Valentina |d 1993- |e VerfasserIn |0 (DE-588)1161434429 |0 (DE-627)1024731324 |0 (DE-576)506521141 |4 aut | |
| 700 | 1 | |a Jänsch, Daniel |e VerfasserIn |0 (DE-588)1157022383 |0 (DE-627)1020019018 |0 (DE-576)50257531X |4 aut | |
| 700 | 1 | |a Freudenberg, Jan |d 1988- |e VerfasserIn |0 (DE-588)1093219564 |0 (DE-627)853188386 |0 (DE-576)462642615 |4 aut | |
| 700 | 1 | |a Beck, Sebastian |d 1985- |e VerfasserIn |0 (DE-588)1063046300 |0 (DE-627)809003570 |0 (DE-576)42038488X |4 aut | |
| 700 | 1 | |a Pucci, Annemarie |e VerfasserIn |0 (DE-588)1020648783 |0 (DE-627)691291969 |0 (DE-576)361698739 |4 aut | |
| 700 | 1 | |a Bunz, Uwe H. F. |d 1963- |e VerfasserIn |0 (DE-588)1080488456 |0 (DE-627)844723223 |0 (DE-576)181112833 |4 aut | |
| 773 | 0 | 8 | |i Enthalten in |t The journal of physical chemistry letters |d Washington, DC : ACS, 2010 |g 9(2018), 13, Seite 3731-3737 |h Online-Ressource |w (DE-627)612168581 |w (DE-600)2522838-9 |w (DE-576)315319089 |x 1948-7185 |7 nnas |a Structure-property relationship of phenylene-based self-assembled monolayers for record low work function of indium tin oxide |
| 773 | 1 | 8 | |g volume:9 |g year:2018 |g number:13 |g pages:3731-3737 |g extent:7 |a Structure-property relationship of phenylene-based self-assembled monolayers for record low work function of indium tin oxide |
| 856 | 4 | 0 | |u https://doi.org/10.1021/acs.jpclett.8b01242 |x Verlag |x Resolving-System |z lizenzpflichtig |3 Volltext |
| 951 | |a AR | ||
| 992 | |a 20200311 | ||
| 993 | |a Article | ||
| 994 | |a 2018 | ||
| 998 | |g 1080488456 |a Bunz, Uwe H. F. |m 1080488456:Bunz, Uwe H. F. |d 120000 |d 120100 |e 120000PB1080488456 |e 120100PB1080488456 |k 0/120000/ |k 1/120000/120100/ |p 12 | ||
| 998 | |g 1020648783 |a Pucci, Annemarie |m 1020648783:Pucci, Annemarie |d 130000 |d 130700 |e 130000PP1020648783 |e 130700PP1020648783 |k 0/130000/ |k 1/130000/130700/ |p 11 | ||
| 998 | |g 1063046300 |a Beck, Sebastian |m 1063046300:Beck, Sebastian |d 130000 |d 130700 |e 130000PB1063046300 |e 130700PB1063046300 |k 0/130000/ |k 1/130000/130700/ |p 8 | ||
| 998 | |g 1093219564 |a Freudenberg, Jan |m 1093219564:Freudenberg, Jan |d 120000 |d 120100 |e 120000PF1093219564 |e 120100PF1093219564 |k 0/120000/ |k 1/120000/120100/ |p 7 | ||
| 998 | |g 1157022383 |a Jänsch, Daniel |m 1157022383:Jänsch, Daniel |d 120000 |d 120100 |e 120000PJ1157022383 |e 120100PJ1157022383 |k 0/120000/ |k 1/120000/120100/ |p 6 | ||
| 998 | |g 1161434429 |a Rohnacher, Valentina |m 1161434429:Rohnacher, Valentina |d 130000 |d 130700 |e 130000PR1161434429 |e 130700PR1161434429 |k 0/130000/ |k 1/130000/130700/ |p 4 | ||
| 998 | |g 107115737X |a Hillebrandt, Sabina |m 107115737X:Hillebrandt, Sabina |d 130000 |d 130700 |e 130000PH107115737X |e 130700PH107115737X |k 0/130000/ |k 1/130000/130700/ |p 2 | ||
| 998 | |g 1194346294 |a Benneckendorf, Frank S. |m 1194346294:Benneckendorf, Frank S. |d 120000 |d 120100 |e 120000PB1194346294 |e 120100PB1194346294 |k 0/120000/ |k 1/120000/120100/ |p 1 |x j | ||
| 999 | |a KXP-PPN1692260901 |e 3606427727 | ||
| BIB | |a Y | ||
| SER | |a journal | ||
| JSO | |a {"title":[{"title_sort":"Structure-property relationship of phenylene-based self-assembled monolayers for record low work function of indium tin oxide","title":"Structure-property relationship of phenylene-based self-assembled monolayers for record low work function of indium tin oxide"}],"person":[{"given":"Frank S.","family":"Benneckendorf","role":"aut","roleDisplay":"VerfasserIn","display":"Benneckendorf, Frank S."},{"role":"aut","display":"Hillebrandt, Sabina","roleDisplay":"VerfasserIn","given":"Sabina","family":"Hillebrandt"},{"roleDisplay":"VerfasserIn","display":"Rohnacher, Valentina","role":"aut","family":"Rohnacher","given":"Valentina"},{"role":"aut","display":"Jänsch, Daniel","roleDisplay":"VerfasserIn","given":"Daniel","family":"Jänsch"},{"given":"Jan","family":"Freudenberg","role":"aut","display":"Freudenberg, Jan","roleDisplay":"VerfasserIn"},{"family":"Beck","given":"Sebastian","display":"Beck, Sebastian","roleDisplay":"VerfasserIn","role":"aut"},{"role":"aut","roleDisplay":"VerfasserIn","display":"Pucci, Annemarie","given":"Annemarie","family":"Pucci"},{"family":"Bunz","given":"Uwe H. F.","display":"Bunz, Uwe H. F.","roleDisplay":"VerfasserIn","role":"aut"}],"note":["Gesehen am 11.03.2020"],"type":{"media":"Online-Ressource","bibl":"article-journal"},"language":["eng"],"recId":"1692260901","origin":[{"dateIssuedDisp":"20 June 2018","dateIssuedKey":"2018"}],"id":{"doi":["10.1021/acs.jpclett.8b01242"],"eki":["1692260901"]},"name":{"displayForm":["Frank S. Benneckendorf, Sabina Hillebrandt, Florian Ullrich, Valentina Rohnacher, Sebastian Hietzschold, Daniel Jänsch, Jan Freudenberg, Sebastian Beck, Eric Mankel, Wolfram Jaegermann, Annemarie Pucci, Uwe H.F. Bunz, and Klaus Müllen"]},"physDesc":[{"extent":"7 S."}],"relHost":[{"pubHistory":["1.2010 -"],"titleAlt":[{"title":"JPCLett"}],"part":{"year":"2018","pages":"3731-3737","issue":"13","volume":"9","text":"9(2018), 13, Seite 3731-3737","extent":"7"},"note":["Gesehen am 02.01.2013"],"disp":"Structure-property relationship of phenylene-based self-assembled monolayers for record low work function of indium tin oxideThe journal of physical chemistry letters","type":{"media":"Online-Ressource","bibl":"periodical"},"language":["eng"],"recId":"612168581","title":[{"title_sort":"journal of physical chemistry letters","title":"The journal of physical chemistry letters"}],"physDesc":[{"extent":"Online-Ressource"}],"origin":[{"publisherPlace":"Washington, DC","dateIssuedDisp":"2010-","dateIssuedKey":"2010","publisher":"ACS"}],"id":{"zdb":["2522838-9"],"eki":["612168581"],"issn":["1948-7185"]},"name":{"displayForm":["American Chemical Society"]}}]} | ||
| SRT | |a BENNECKENDSTRUCTUREP2020 | ||