Oxygen-catalysed sequential singlet fission
Singlet fission is a promising carrier multiplication process, where a singlet exciton is split in two triplet states. Here the authors propose an oxygen-assisted two-step mechanism for singlet fission accounting for ~ 40% triplet quantum yield in dilute solutions where the single-step mechanism is...
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| Hauptverfasser: | , , , , |
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| Dokumenttyp: | Article (Journal) |
| Sprache: | Englisch |
| Veröffentlicht: |
15 November 2019
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| In: |
Nature Communications
Year: 2019, Jahrgang: 10 |
| ISSN: | 2041-1723 |
| DOI: | 10.1038/s41467-019-13202-5 |
| Online-Zugang: | Verlag, lizenzpflichtig, Volltext: https://doi.org/10.1038/s41467-019-13202-5 Verlag, lizenzpflichtig, Volltext: https://www.nature.com/articles/s41467-019-13202-5 |
| Verfasserangaben: | Nikolaus Wollscheid, J. Luis Pérez Lustres, Oskar Kefer, Sebastian Hahn, Victor Brosius, Uwe H.F. Bunz, Marcus Motzkus & Tiago Buckup |
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| 520 | |a Singlet fission is a promising carrier multiplication process, where a singlet exciton is split in two triplet states. Here the authors propose an oxygen-assisted two-step mechanism for singlet fission accounting for ~ 40% triplet quantum yield in dilute solutions where the single-step mechanism is inactive. | ||
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