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Intermolecular Coulombic decay in endohedral fullerene at the 4d → 4f resonance

Intermolecular processes offer unique decay mechanisms for complex systems to internally relax. Here, we report the observation of an intermolecular Coulombic decay channel in an endohedral fullerene, a holmium nitride complex (Ho3N) embedded within a C80 fullerene, between neighboring holmium ions,...

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Hauptverfasser: Obaid, Razib (VerfasserIn) , Xiong, Hui (VerfasserIn) , Augustin, Sven (VerfasserIn) , Schnorr, Kirsten (VerfasserIn) , Ablikim, Utuq (VerfasserIn) , Battistoni, Andrea (VerfasserIn) , Wolf, Thomas J. A. (VerfasserIn) , Bilodeau, René C. (VerfasserIn) , Osipov, Timur (VerfasserIn) , Gokhberg, Kirill (VerfasserIn) , Rolles, Daniel (VerfasserIn) , LaForge, Aaron C. (VerfasserIn) , Berrah, Nora (VerfasserIn)
Dokumenttyp: Article (Journal)
Sprache:Englisch
Veröffentlicht: 17 March 2020
In: Physical review letters
Year: 2020, Jahrgang: 124, Heft: 11
ISSN:1079-7114
DOI:10.1103/PhysRevLett.124.113002
Online-Zugang:Verlag, lizenzpflichtig, Volltext: https://doi.org/10.1103/PhysRevLett.124.113002
Verlag, lizenzpflichtig, Volltext: https://link.aps.org/doi/10.1103/PhysRevLett.124.113002
Volltext
Verfasserangaben:Razib Obaid, Hui Xiong, Sven Augustin, Kirsten Schnorr, Utuq Ablikim, Andrea Battistoni, Thomas J.A. Wolf, René C. Bilodeau, Timur Osipov, Kirill Gokhberg, Daniel Rolles, Aaron C. LaForge, and Nora Berrah
Beschreibung
Zusammenfassung:Intermolecular processes offer unique decay mechanisms for complex systems to internally relax. Here, we report the observation of an intermolecular Coulombic decay channel in an endohedral fullerene, a holmium nitride complex (Ho3N) embedded within a C80 fullerene, between neighboring holmium ions, and between the holmium complex and the carbon cage. By measuring the ions and the electrons in coincidence after XUV photoabsorption, we can isolate the different decay channels, which are found to be more prevalent relative to intra-atomic Auger decay.
Beschreibung:Gesehen am 30.04.2020
Beschreibung:Online Resource
ISSN:1079-7114
DOI:10.1103/PhysRevLett.124.113002

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