Trion-Polariton formation in single-walled carbon nanotube microcavities
We demonstrate the formation and tuning of charged trion-polaritons in polymer-sorted (6,5) single-walled carbon nanotubes in a planar metal-clad microcavity at room temperature. The positively charged trion-polaritons were induced by electrochemical doping and characterized by angle-resolved reflec...
Gespeichert in:
| Hauptverfasser: | , , , , , |
|---|---|
| Dokumenttyp: | Article (Journal) |
| Sprache: | Englisch |
| Veröffentlicht: |
8 May 2018
|
| In: |
ACS photonics
Year: 2018, Jahrgang: 5, Heft: 6, Pages: 2074-2080 |
| ISSN: | 2330-4022 |
| DOI: | 10.1021/acsphotonics.7b01549 |
| Online-Zugang: | Verlag, lizenzpflichtig, Volltext: https://doi.org/10.1021/acsphotonics.7b01549
|
| Verfasserangaben: | Charles Möhl, Arko Graf, Felix J. Berger, Jan Lüttgens, Yuriy Zakharko, Victoria Lumsargis, Malte C. Gather, and Jana Zaumseil |
| Zusammenfassung: | We demonstrate the formation and tuning of charged trion-polaritons in polymer-sorted (6,5) single-walled carbon nanotubes in a planar metal-clad microcavity at room temperature. The positively charged trion-polaritons were induced by electrochemical doping and characterized by angle-resolved reflectance and photoluminescence spectroscopy. The doping level of the nanotubes within the microcavity was controlled by the applied bias and thus enabled tuning from mainly excitonic to a mixture of exciton and trion transitions. Mode splitting of more than 70 meV around the trion energy and emission from the new lower polariton branch corroborate a transition from exciton-polaritons (neutral) to trion-polaritons (charged). The estimated charge-to-mass ratio of these trion-polaritons is 200 times higher than that of electrons or holes in carbon nanotubes, which has exciting implications for the realization of polaritonic charge transport. |
|---|---|
| Beschreibung: | Gesehen am 06.05.2020 |
| Beschreibung: | Online Resource |
| ISSN: | 2330-4022 |
| DOI: | 10.1021/acsphotonics.7b01549 |