Trion-Polariton formation in single-walled carbon nanotube microcavities
We demonstrate the formation and tuning of charged trion-polaritons in polymer-sorted (6,5) single-walled carbon nanotubes in a planar metal-clad microcavity at room temperature. The positively charged trion-polaritons were induced by electrochemical doping and characterized by angle-resolved reflec...
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| Main Authors: | , , , , , |
|---|---|
| Format: | Article (Journal) |
| Language: | English |
| Published: |
8 May 2018
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| In: |
ACS photonics
Year: 2018, Volume: 5, Issue: 6, Pages: 2074-2080 |
| ISSN: | 2330-4022 |
| DOI: | 10.1021/acsphotonics.7b01549 |
| Online Access: | Verlag, lizenzpflichtig, Volltext: https://doi.org/10.1021/acsphotonics.7b01549
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| Author Notes: | Charles Möhl, Arko Graf, Felix J. Berger, Jan Lüttgens, Yuriy Zakharko, Victoria Lumsargis, Malte C. Gather, and Jana Zaumseil |
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| 520 | |a We demonstrate the formation and tuning of charged trion-polaritons in polymer-sorted (6,5) single-walled carbon nanotubes in a planar metal-clad microcavity at room temperature. The positively charged trion-polaritons were induced by electrochemical doping and characterized by angle-resolved reflectance and photoluminescence spectroscopy. The doping level of the nanotubes within the microcavity was controlled by the applied bias and thus enabled tuning from mainly excitonic to a mixture of exciton and trion transitions. Mode splitting of more than 70 meV around the trion energy and emission from the new lower polariton branch corroborate a transition from exciton-polaritons (neutral) to trion-polaritons (charged). The estimated charge-to-mass ratio of these trion-polaritons is 200 times higher than that of electrons or holes in carbon nanotubes, which has exciting implications for the realization of polaritonic charge transport. | ||
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