Photo-cross-linkable polymeric optoelectronics based on the [2 + 2] cycloaddition reaction of cinnamic acid
We report the synthesis of cinnamic acid-functionalized conjugated polymers, which are cross-linked via [2 + 2] cycloaddition by UV illumination, reducing their solubility. The cross-linking reaction was investigated by a combination of FTIR and optical spectroscopy, and an optimum condition for the...
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| Hauptverfasser: | , , , , , , , , , , |
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| Dokumenttyp: | Article (Journal) |
| Sprache: | Englisch |
| Veröffentlicht: |
February 16, 2016
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| In: |
Macromolecules
Year: 2016, Jahrgang: 49, Heft: 5, Pages: 1518-1522 |
| ISSN: | 1520-5835 |
| DOI: | 10.1021/acs.macromol.5b02407 |
| Online-Zugang: | Resolving-System, lizenzpflichtig, Volltext: https://doi.org/10.1021/acs.macromol.5b02407 Verlag, lizenzpflichtig, Volltext: https://pubs.acs.org/doi/10.1021/acs.macromol.5b02407 
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| Verfasserangaben: | Korwin M. Schelkle, Markus Bender, Sebastian Beck, Krischan F. Jeltsch, Sebastian Stolz, Johannes Zimmermann, R. Thomas Weitz, Annemarie Pucci, Klaus Müllen, Manuel Hamburger, and Uwe H. F. Bunz |
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| 520 | |a We report the synthesis of cinnamic acid-functionalized conjugated polymers, which are cross-linked via [2 + 2] cycloaddition by UV illumination, reducing their solubility. The cross-linking reaction was investigated by a combination of FTIR and optical spectroscopy, and an optimum condition for the solubility modulation of thin films, a major challenge in the solution-phase fabrication of layered optoelectronic devices, was reached. As proof of concept, OLEDs were fabricated, using these conjugated polymers as emissive layers. | ||
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