Static and dynamic magnetic response of fragmented haldane-like spin chains in layered Li3Cu2SbO6
The structure and the magnetic properties of layered Li3Cu2SbO6 are investigated by powder X-ray diffraction, static susceptibility, and electron spin resonance studies up to 330 GHz. The XRD data experimentally verify the space group C2/m with halved unit cell volume in contrast to previously repor...
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| Hauptverfasser: | , |
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| Dokumenttyp: | Article (Journal) |
| Sprache: | Englisch |
| Veröffentlicht: |
July 11, 2016
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| In: |
Journal of the Physical Society of Japan
Year: 2016, Jahrgang: 85, Heft: 8, Pages: ? |
| ISSN: | 1347-4073 |
| DOI: | 10.7566/JPSJ.85.084702 |
| Online-Zugang: | Verlag, lizenzpflichtig, Volltext: https://doi.org/10.7566/JPSJ.85.084702 Verlag, lizenzpflichtig, Volltext: https://journals.jps.jp/doi/10.7566/JPSJ.85.084702 
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| Verfasserangaben: | Changhyun Koo, Elena A. Zvereva, Igor L. Shukaev, Michael Richter, Mikhail I. Stratan, Alexander N. Vasiliev, Vladimir B. Nalbandyan, and Rüdiger Klingeler |
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| 245 | 1 | 0 | |a Static and dynamic magnetic response of fragmented haldane-like spin chains in layered Li3Cu2SbO6 |c Changhyun Koo, Elena A. Zvereva, Igor L. Shukaev, Michael Richter, Mikhail I. Stratan, Alexander N. Vasiliev, Vladimir B. Nalbandyan, and Rüdiger Klingeler |
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| 520 | |a The structure and the magnetic properties of layered Li3Cu2SbO6 are investigated by powder X-ray diffraction, static susceptibility, and electron spin resonance studies up to 330 GHz. The XRD data experimentally verify the space group C2/m with halved unit cell volume in contrast to previously reported C2/c. In addition, the data show significant Li/Cu-intersite exchange. Static magnetic susceptibility and ESR measurements show two magnetic contributions, i.e., quasi-free spins at low-temperature and a spin-gapped magnetic subsystem, with about half of the spins being associated to each subsystem. The data suggest ferromagnetic-antiferromagnetic alternating chains with JFM = −285 K and JAFM = 160 K with a significant amount of Li-defects in the chains. The results are discussed in the scenario of fragmented 1D S = 1 AFM chains with a rather high defect concentration of about 17% and associated S = 1/2 edge states of the resulting finite Haldane chains. | ||
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