One-step additive crosslinking of conjugated polyelectrolyte interlayers: improved lifetime and performance of solution-processed OLEDs
We crosslink an amino-functionalized polyfluorene by the solvent additive 1,8-diiodooctane (DIO). DIO remains in the film after drying of the main solvent and chemically binds to the amino-side groups after a low temperature annealing step, rendering the polyfluorene film insoluble in non-polar solv...
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| Hauptverfasser: | , , , , , |
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| Dokumenttyp: | Article (Journal) |
| Sprache: | Englisch |
| Veröffentlicht: |
08 Nov 2016
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| In: |
Journal of materials chemistry. C, Materials for optical and electronic devices
Year: 2016, Jahrgang: 4, Heft: 47, Pages: 11150-11156 |
| ISSN: | 2050-7534 |
| DOI: | 10.1039/C6TC04417D |
| Online-Zugang: | Verlag, lizenzpflichtig, Volltext: https://doi.org/10.1039/C6TC04417D Verlag, lizenzpflichtig, Volltext: https://pubs.rsc.org/en/content/articlelanding/2016/tc/c6tc04417d 
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| Verfasserangaben: | Sebastian Stolz, Martin Petzoldt, Naresh Kotadiya, Tobias Rödlmeier, Ralph Eckstein, Jan Freudenberg, Uwe H.F. Bunz, Uli Lemmer, Eric Mankel, Manuel Hamburger and Gerardo Hernandez-Sosa |
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| 520 | |a We crosslink an amino-functionalized polyfluorene by the solvent additive 1,8-diiodooctane (DIO). DIO remains in the film after drying of the main solvent and chemically binds to the amino-side groups after a low temperature annealing step, rendering the polyfluorene film insoluble in non-polar solvents. We correlate the amount of DIO, the reduction of operational voltage and increase in lifetime of solution-processed OLEDs. We demonstrate a fully solution-processed device using the crosslinked polyfluorene electron injection layer and an inkjet-printed Ag top electrode. | ||
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