Magnetic anisotropy and the phase diagram of chiral MnSb2O6

The magnetic phase diagram and low-energy magnon excitations of structurally and magnetically chiral MnSb2O6 are reported. The specific heat and the static magnetization are investigated in magnetic fields up to 9 and 30 T, respectively, while the dynamic magnetic properties are probed by X-band as...

Ausführliche Beschreibung

Gespeichert in:
Bibliographische Detailangaben
Hauptverfasser: Werner, Johannes (VerfasserIn) , Koo, Changhyun (VerfasserIn) , Klingeler, Rüdiger (VerfasserIn)
Dokumenttyp: Article (Journal)
Sprache:Englisch
Veröffentlicht: 6 September 2016
In: Physical review
Year: 2016, Jahrgang: 94, Heft: 10
ISSN:2469-9969
DOI:10.1103/PhysRevB.94.104408
Online-Zugang:Verlag, lizenzpflichtig, Volltext: https://doi.org/10.1103/PhysRevB.94.104408
Verlag, lizenzpflichtig, Volltext: https://link.aps.org/doi/10.1103/PhysRevB.94.104408
Volltext
Verfasserangaben:J. Werner, C. Koo, R. Klingeler, A.N. Vasiliev, Y.A. Ovchenkov, A.S. Polovkova, G.V. Raganyan, E.A. Zvereva
Beschreibung
Zusammenfassung:The magnetic phase diagram and low-energy magnon excitations of structurally and magnetically chiral MnSb2O6 are reported. The specific heat and the static magnetization are investigated in magnetic fields up to 9 and 30 T, respectively, while the dynamic magnetic properties are probed by X-band as well as tunable high-frequency electron spin-resonance spectroscopy. Below TN=11.5 K, we observe antiferromagnetic resonance modes which imply small but finite planar anisotropy showing up in a zero-field splitting of 20 GHz. The data are well described by means of an easy-plane two-sublattice model with the anisotropy field BA=0.02 T. The exchange field BE=13 T is obtained from the saturation field derived from the pulsed-field magnetization. A crucial role of the small anisotropy for the spin structure is reflected by competing antiferromagnetic phases appearing, at T=2 K, in small magnetic fields at BC1 ≈0.5 T and BC2=0.9 T. We discuss the results in terms of spin reorientation and of small magnetic fields favoring helical spin structure over the cycloidal ground state which, at B=0, is stabilized by the planar anisotropy. Above TN, short-range magnetic correlations up to ≳60 K and magnetic entropy changes well above TN reflect the frustrated triangular arrangement of Mn2+ ions in MnSb2O6.
Beschreibung:Im Titel ist die Zahl "2" und "6" tiefgestellt
Beschreibung:Online Resource
ISSN:2469-9969
DOI:10.1103/PhysRevB.94.104408