N,N′-dihydrotetraazapentacenes (DHTA) in thin film transistors
The synthesis and structural properties of three N,N′-dihydrotetraazapentacenes (DHTA) are described. The different substitution pattern (H, F, Cl) of the dihydrotetraazapentacene body exhibited a significant effect on the optical, electronic and morphological properties of the derivatives in thin f...
Gespeichert in:
| Hauptverfasser: | , , , , , , , |
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| Dokumenttyp: | Article (Journal) |
| Sprache: | Englisch |
| Veröffentlicht: |
2015
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| In: |
Journal of materials chemistry. C, Materials for optical and electronic devices
Year: 2015, Jahrgang: 3, Heft: 7, Pages: 1604-1609 |
| ISSN: | 2050-7534 |
| DOI: | 10.1039/C4TC02426E |
| Online-Zugang: | Verlag, lizenzpflichtig, Volltext: https://doi.org/10.1039/C4TC02426E Verlag, lizenzpflichtig, Volltext: https://pubs.rsc.org/en/content/articlelanding/2015/tc/c4tc02426e 
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| Verfasserangaben: | Fabian Paulus, Benjamin D. Lindner, Hilmar Reiß, Frank Rominger, Andreas Leineweber, Yana Vaynzof, Henning Sirringhaus and Uwe H.F. Bunz |
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| 520 | |a The synthesis and structural properties of three N,N′-dihydrotetraazapentacenes (DHTA) are described. The different substitution pattern (H, F, Cl) of the dihydrotetraazapentacene body exhibited a significant effect on the optical, electronic and morphological properties of the derivatives in thin films. The synthesised materials were investigated as active layers in top gate/bottom contact (BC/TG) transistors. The transistor performance of the dichlorinated derivative was almost independent on the processing conditions with an average hole mobility of ∼0.04 cm2 V−1 s−1 and best mobility values ranging from 0.07 to 0.11 cm2 V−1 s−1. Each of the three derivatives was found to exhibit an individual packing motif in solution grown crystals, determined by single crystal X-ray analysis. Surprisingly, for all three materials a different polymorph formed in spin cast films explaining the observed morphology and FET performance. | ||
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