Nonlinear optical response of photochromic azobenzene-functionalized self-assembled monolayers
The combination of photochromic and nonlinear optical (NLO) properties of azobenzene-functionalized self-assembled monolayers (SAMs) constitutes an intriguing step towards novel photonic and optoelectronic devices. By utilizing the second-order NLO process of second harmonic generation (SHG), suppor...
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| Hauptverfasser: | , , , , , , , |
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| Dokumenttyp: | Article (Journal) |
| Sprache: | Englisch |
| Veröffentlicht: |
18 June 2015
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| In: |
Physical chemistry, chemical physics
Year: 2015, Jahrgang: 17, Heft: 27, Pages: 18079-18086 |
| ISSN: | 1463-9084 |
| DOI: | 10.1039/C5CP03093E |
| Online-Zugang: | Verlag, lizenzpflichtig, Volltext: https://doi.org/10.1039/C5CP03093E Verlag, lizenzpflichtig, Volltext: https://pubs.rsc.org/en/content/articlelanding/2015/cp/c5cp03093e 
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| Verfasserangaben: | Michael Schulze, Manuel Utecht, Thomas Moldt, Daniel Przyrembel, Cornelius Gahl, Martin Weinelt, Peter Saalfrank and Petra Tegeder |
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| 520 | |a The combination of photochromic and nonlinear optical (NLO) properties of azobenzene-functionalized self-assembled monolayers (SAMs) constitutes an intriguing step towards novel photonic and optoelectronic devices. By utilizing the second-order NLO process of second harmonic generation (SHG), supported by density-functional theory and correlated wave function method calculations, we demonstrate that the photochromic interface provides the necessary prerequisites en route towards possible future technical applications: we find a high NLO contrast on the order of 16% between the switching states. These are furthermore accessible reversibly and with high efficiencies in terms of cross sections on the order of 10−18 cm2 for both photoisomerization reactions, i.e., drivable by means of low-power LED light sources. Finally, both photostationary states (PSSs) are thermally stable at ambient conditions. | ||
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