On-surface synthesis of a two-dimensional porous coordination network: Unraveling adsorbate interactions
We present a detailed experimental and theoretical characterization of the adsorption of the perylene derivative 4,9-diaminoperylene-quinone-3,10-diimine (DPDI) on Cu(111) and compare it to its threefold dehydrogenated derivative 3deh-DPDI, which forms in a surface reaction upon annealing. While DPD...
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| Main Authors: | , , , , , , , , |
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| Format: | Article (Journal) |
| Language: | English |
| Published: |
5 September 2014
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| In: |
Physical review. B, Condensed matter and materials physics
Year: 2014, Volume: 90, Issue: 12 |
| ISSN: | 1550-235X |
| DOI: | 10.1103/PhysRevB.90.125408 |
| Online Access: | Verlag, lizenzpflichtig, Volltext: https://doi.org/10.1103/PhysRevB.90.125408 Verlag, lizenzpflichtig, Volltext: https://link.aps.org/doi/10.1103/PhysRevB.90.125408 
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| Author Notes: | Manfred Matena, Jonas Björk, Markus Wahl, Tien-Lin Lee, Jörg Zegenhagen, Lutz H. Gade, Thomas A. Jung, Mats Persson, and Meike Stöhr |
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| 245 | 1 | 0 | |a On-surface synthesis of a two-dimensional porous coordination network |b Unraveling adsorbate interactions |c Manfred Matena, Jonas Björk, Markus Wahl, Tien-Lin Lee, Jörg Zegenhagen, Lutz H. Gade, Thomas A. Jung, Mats Persson, and Meike Stöhr |
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| 520 | |a We present a detailed experimental and theoretical characterization of the adsorption of the perylene derivative 4,9-diaminoperylene-quinone-3,10-diimine (DPDI) on Cu(111) and compare it to its threefold dehydrogenated derivative 3deh-DPDI, which forms in a surface reaction upon annealing. While DPDI itself does not give rise to long-range ordered structures due to lack of appropriate functional groups, 3deh-DPDI acts as an exoligand in a Cu-coordinated honeycomb network on Cu(111). The main focus of this work lies on the analysis of intermolecular and molecule-substrate interactions by combining results from scanning tunneling microscopy, x-ray photoelectron spectroscopy, x-ray standing wave measurements, and density functional theory. We show, in particular, that the interactions between metal atoms and organic ligands effectively weaken the molecule-surface interactions for 3deh-DPDI leading to an increase in molecule-substrate distances compared to the DPDI precursor. Our experimental findings also shed light on the applicability of current theories, namely van der Waals corrections to density functional theory. | ||
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| 700 | 1 | |a Wahl, Markus |e VerfasserIn |4 aut | |
| 700 | 1 | |a Lee, Tien-Lin |e VerfasserIn |4 aut | |
| 700 | 1 | |a Zegenhagen, Jörg |e VerfasserIn |4 aut | |
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| 700 | 1 | |a Jung, Thomas A. |e VerfasserIn |4 aut | |
| 700 | 1 | |a Persson, Mats |e VerfasserIn |4 aut | |
| 700 | 1 | |a Stöhr, Meike |e VerfasserIn |4 aut | |
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