Buchumschlag

Quantum effects dominating the interatomic coulombic decay of an extreme system

LiHe is an extreme open-shell system. It is among the weakest bound systems known, and its mean interatomic distance extends dramatically into the classical forbidden region. Upon 1s → 2p excitation of He, interatomic Coulombic decay (ICD) takes place in which the electronically excited helium atom...

Ausführliche Beschreibung

Gespeichert in:
Bibliographische Detailangaben
Hauptverfasser: Ben-Asher, Anael (VerfasserIn) , Landau, Arik (VerfasserIn) , Cederbaum, Lorenz S. (VerfasserIn) , Moiseyev, Nimrod (VerfasserIn)
Dokumenttyp: Article (Journal)
Sprache:Englisch
Veröffentlicht: July 24, 2020
In: The journal of physical chemistry letters
Year: 2020, Jahrgang: 11, Heft: 16, Pages: 6600-6605
ISSN:1948-7185
DOI:10.1021/acs.jpclett.0c01974
Online-Zugang:Verlag, lizenzpflichtig, Volltext: https://doi.org/10.1021/acs.jpclett.0c01974
Volltext
Verfasserangaben:Anael Ben-Asher, Arie Landau, Lorenz S. Cederbaum, and Nimrod Moiseyev

MARC

LEADER 00000caa a2200000 c 4500
001 1734608943
003 DE-627
005 20230427033705.0
007 cr uuu---uuuuu
008 201005s2020 xx |||||o 00| ||eng c
024 7 |a 10.1021/acs.jpclett.0c01974  |2 doi 
035 |a (DE-627)1734608943 
035 |a (DE-599)KXP1734608943 
035 |a (OCoLC)1341368367 
040 |a DE-627  |b ger  |c DE-627  |e rda 
041 |a eng 
084 |a 30  |2 sdnb 
100 1 |a Ben-Asher, Anael  |e VerfasserIn  |0 (DE-588)1218978872  |0 (DE-627)1734609826  |4 aut 
245 1 0 |a Quantum effects dominating the interatomic coulombic decay of an extreme system  |c Anael Ben-Asher, Arie Landau, Lorenz S. Cederbaum, and Nimrod Moiseyev 
264 1 |c July 24, 2020 
300 |a 6 
336 |a Text  |b txt  |2 rdacontent 
337 |a Computermedien  |b c  |2 rdamedia 
338 |a Online-Ressource  |b cr  |2 rdacarrier 
500 |a Gesehen am 05.10.2020 
520 |a LiHe is an extreme open-shell system. It is among the weakest bound systems known, and its mean interatomic distance extends dramatically into the classical forbidden region. Upon 1s → 2p excitation of He, interatomic Coulombic decay (ICD) takes place in which the electronically excited helium atom relaxes and transfers its excess energy to ionize the neighboring lithium atom. A substantial part of the decay is found to be to the dissociation continuum producing Li+ and He atoms. The distribution of the kinetic energy released by the ICD products is found to be highly oscillatory. Its analysis reveals that quantum phase shifts between the decaying states and the dissociating final states are controlling this ICD reaction. The semiclassical reflection principle, which commonly explains ICD reactions, fails. The process is expected to be amenable to experiment. 
700 1 |a Landau, Arik  |e VerfasserIn  |0 (DE-588)1211506738  |0 (DE-627)169978339X  |4 aut 
700 1 |a Cederbaum, Lorenz S.  |d 1946-  |e VerfasserIn  |0 (DE-588)172484952  |0 (DE-627)697422798  |0 (DE-576)133346145  |4 aut 
700 1 |a Moiseyev, Nimrod  |d 1947-  |e VerfasserIn  |0 (DE-588)1011485613  |0 (DE-627)658854607  |0 (DE-576)170876535  |4 aut 
773 0 8 |i Enthalten in  |t The journal of physical chemistry letters  |d Washington, DC : ACS, 2010  |g 11(2020), 16, Seite 6600-6605  |h Online-Ressource  |w (DE-627)612168581  |w (DE-600)2522838-9  |w (DE-576)315319089  |x 1948-7185  |7 nnas  |a Quantum effects dominating the interatomic coulombic decay of an extreme system 
773 1 8 |g volume:11  |g year:2020  |g number:16  |g pages:6600-6605  |g extent:6  |a Quantum effects dominating the interatomic coulombic decay of an extreme system 
856 4 0 |u https://doi.org/10.1021/acs.jpclett.0c01974  |x Verlag  |x Resolving-System  |z lizenzpflichtig  |3 Volltext 
951 |a AR 
992 |a 20201005 
993 |a Article 
994 |a 2020 
998 |g 172484952  |a Cederbaum, Lorenz S.  |m 172484952:Cederbaum, Lorenz S.  |d 120000  |d 120300  |e 120000PC172484952  |e 120300PC172484952  |k 0/120000/  |k 1/120000/120300/  |p 3 
998 |g 1211506738  |a Landau, Arik  |m 1211506738:Landau, Arik  |d 120000  |d 120300  |e 120000PL1211506738  |e 120300PL1211506738  |k 0/120000/  |k 1/120000/120300/  |p 2 
999 |a KXP-PPN1734608943  |e 3766872133 
BIB |a Y 
SER |a journal 
JSO |a {"name":{"displayForm":["Anael Ben-Asher, Arie Landau, Lorenz S. Cederbaum, and Nimrod Moiseyev"]},"person":[{"role":"aut","roleDisplay":"VerfasserIn","family":"Ben-Asher","display":"Ben-Asher, Anael","given":"Anael"},{"given":"Arik","display":"Landau, Arik","family":"Landau","roleDisplay":"VerfasserIn","role":"aut"},{"roleDisplay":"VerfasserIn","role":"aut","family":"Cederbaum","given":"Lorenz S.","display":"Cederbaum, Lorenz S."},{"given":"Nimrod","display":"Moiseyev, Nimrod","roleDisplay":"VerfasserIn","role":"aut","family":"Moiseyev"}],"title":[{"title":"Quantum effects dominating the interatomic coulombic decay of an extreme system","title_sort":"Quantum effects dominating the interatomic coulombic decay of an extreme system"}],"physDesc":[{"extent":"6 S."}],"language":["eng"],"recId":"1734608943","id":{"eki":["1734608943"],"doi":["10.1021/acs.jpclett.0c01974"]},"origin":[{"dateIssuedKey":"2020","dateIssuedDisp":"July 24, 2020"}],"relHost":[{"id":{"issn":["1948-7185"],"eki":["612168581"],"zdb":["2522838-9"]},"recId":"612168581","physDesc":[{"extent":"Online-Ressource"}],"language":["eng"],"note":["Gesehen am 02.01.2013"],"type":{"bibl":"periodical","media":"Online-Ressource"},"pubHistory":["1.2010 -"],"origin":[{"publisherPlace":"Washington, DC","dateIssuedDisp":"2010-","dateIssuedKey":"2010","publisher":"ACS"}],"part":{"volume":"11","issue":"16","extent":"6","pages":"6600-6605","text":"11(2020), 16, Seite 6600-6605","year":"2020"},"titleAlt":[{"title":"JPCLett"}],"name":{"displayForm":["American Chemical Society"]},"disp":"Quantum effects dominating the interatomic coulombic decay of an extreme systemThe journal of physical chemistry letters","title":[{"title":"The journal of physical chemistry letters","title_sort":"journal of physical chemistry letters"}]}],"type":{"bibl":"article-journal","media":"Online-Ressource"},"note":["Gesehen am 05.10.2020"]} 
SRT |a BENASHERANQUANTUMEFF2420 

Ähnliche Einträge