Electron dynamics of interatomic Coulombic decay in quantum dots induced by a laser field

In this paper we investigated the dynamics of an electron in the presence of a time-dependent laser field in a model potential for a two-level single-electron semiconductor quantum dot (QD) that is capable of undergoing interatomic Coulombic decay (ICD) together with an electron bound to a neighbori...

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Bibliographic Details
Main Author: Bande, Annika (Author)
Format: Article (Journal)
Language:English
Published: 4 June 2013
In: The journal of chemical physics
Year: 2013, Volume: 138, Issue: 21
ISSN:1089-7690
DOI:10.1063/1.4807611
Online Access:Verlag, lizenzpflichtig, Volltext: https://doi.org/10.1063/1.4807611
Verlag, lizenzpflichtig, Volltext: https://aip.scitation.org/doi/10.1063/1.4807611
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Author Notes:Annika Bande

MARC

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520 |a In this paper we investigated the dynamics of an electron in the presence of a time-dependent laser field in a model potential for a two-level single-electron semiconductor quantum dot (QD) that is capable of undergoing interatomic Coulombic decay (ICD) together with an electron bound to a neighboring QD. We demonstrate that ICD can be initiated by coupling the two-level QD to either a continuous or a pulsed moderate to strong laser and we obtain the total and partial decay widths of the resonance excited state in agreement with that from the solely decay of the resonance [A. Bande, K. Gokhberg, and L. S. Cederbaum, J. Chem. Phys. 135, 144112 (2011) https://doi.org/10.1063/1.3646205.]. A detailed discussion of the effects of direct ionization by the laser in single- or multi-photon process as well as Rabi oscillations is furthermore presented. 
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