Coherent high-frequency vibrational dynamics in the excited electronic state of all-trans retinal derivatives
Coherent vibrational dynamics of retinal in excited electronic states are of primary importance in the understanding of photobiology. Using pump-DFWM, we demonstrate for the first time the existence of coherent double-bond high-frequency modulations (>1300 cm-1) in the excited electronic state of...
Saved in:
| Main Authors: | , , |
|---|---|
| Format: | Article (Journal) |
| Language: | English |
| Published: |
January 10, 2013
|
| In: |
The journal of physical chemistry letters
Year: 2013, Volume: 4, Issue: 3, Pages: 383-387 |
| ISSN: | 1948-7185 |
| DOI: | 10.1021/jz302001m |
| Online Access: | Verlag, lizenzpflichtig, Volltext: https://doi.org/10.1021/jz302001m |
| Author Notes: | Jan Philip Kraack, Tiago Buckup, and Marcus Motzkus |
MARC
| LEADER | 00000caa a2200000 c 4500 | ||
|---|---|---|---|
| 001 | 175258371X | ||
| 003 | DE-627 | ||
| 005 | 20230427070822.0 | ||
| 007 | cr uuu---uuuuu | ||
| 008 | 210326s2013 xx |||||o 00| ||eng c | ||
| 024 | 7 | |a 10.1021/jz302001m |2 doi | |
| 035 | |a (DE-627)175258371X | ||
| 035 | |a (DE-599)KXP175258371X | ||
| 035 | |a (OCoLC)1341401487 | ||
| 040 | |a DE-627 |b ger |c DE-627 |e rda | ||
| 041 | |a eng | ||
| 084 | |a 30 |2 sdnb | ||
| 100 | 1 | |a Kraack, Jan Philip |e VerfasserIn |0 (DE-588)1051449693 |0 (DE-627)78630670X |0 (DE-576)406529604 |4 aut | |
| 245 | 1 | 0 | |a Coherent high-frequency vibrational dynamics in the excited electronic state of all-trans retinal derivatives |c Jan Philip Kraack, Tiago Buckup, and Marcus Motzkus |
| 264 | 1 | |c January 10, 2013 | |
| 300 | |a 5 | ||
| 336 | |a Text |b txt |2 rdacontent | ||
| 337 | |a Computermedien |b c |2 rdamedia | ||
| 338 | |a Online-Ressource |b cr |2 rdacarrier | ||
| 500 | |a Gesehen am 04.11.2021 | ||
| 520 | |a Coherent vibrational dynamics of retinal in excited electronic states are of primary importance in the understanding of photobiology. Using pump-DFWM, we demonstrate for the first time the existence of coherent double-bond high-frequency modulations (>1300 cm-1) in the excited electronic state of different retinal derivatives. All-trans retinal as well as retinal Schiff bases exhibit a partial frequency downshift of the C═C double-bond mode from ∼1580 cm-1 in the ground state to 1510 cm-1 in the excited state. In addition, a new vibrational band at ∼1700 cm-1 assigned to the C═N stretching mode in retinal Schiff bases in the excited state is detected. The newly reported bands are observed only in specific spectral regions of excited-state absorption. Implications regarding the observation of vibrational coherences in naturally occurring retinal protonated Schiff bases in rhodopsins are discussed. | ||
| 700 | 1 | |a Buckup, Tiago |d 1976- |e VerfasserIn |0 (DE-588)1080491090 |0 (DE-627)844732893 |0 (DE-576)453560830 |4 aut | |
| 700 | 1 | |a Motzkus, Marcus |e VerfasserIn |0 (DE-588)1080500839 |0 (DE-627)844734020 |0 (DE-576)453561551 |4 aut | |
| 773 | 0 | 8 | |i Enthalten in |t The journal of physical chemistry letters |d Washington, DC : ACS, 2010 |g 4(2013), 3, Seite 383-387 |h Online-Ressource |w (DE-627)612168581 |w (DE-600)2522838-9 |w (DE-576)315319089 |x 1948-7185 |7 nnas |a Coherent high-frequency vibrational dynamics in the excited electronic state of all-trans retinal derivatives |
| 773 | 1 | 8 | |g volume:4 |g year:2013 |g number:3 |g pages:383-387 |g extent:5 |a Coherent high-frequency vibrational dynamics in the excited electronic state of all-trans retinal derivatives |
| 856 | 4 | 0 | |u https://doi.org/10.1021/jz302001m |x Verlag |x Resolving-System |z lizenzpflichtig |3 Volltext |
| 951 | |a AR | ||
| 992 | |a 20210326 | ||
| 993 | |a Article | ||
| 994 | |a 2013 | ||
| 998 | |g 1080500839 |a Motzkus, Marcus |m 1080500839:Motzkus, Marcus |d 120000 |d 120300 |e 120000PM1080500839 |e 120300PM1080500839 |k 0/120000/ |k 1/120000/120300/ |p 3 |y j | ||
| 998 | |g 1080491090 |a Buckup, Tiago |m 1080491090:Buckup, Tiago |d 120000 |d 120300 |e 120000PB1080491090 |e 120300PB1080491090 |k 0/120000/ |k 1/120000/120300/ |p 2 | ||
| 998 | |g 1051449693 |a Kraack, Jan Philip |m 1051449693:Kraack, Jan Philip |d 120000 |e 120000PK1051449693 |k 0/120000/ |p 1 |x j | ||
| 999 | |a KXP-PPN175258371X |e 3894826819 | ||
| BIB | |a Y | ||
| SER | |a journal | ||
| JSO | |a {"type":{"media":"Online-Ressource","bibl":"article-journal"},"note":["Gesehen am 04.11.2021"],"language":["eng"],"recId":"175258371X","person":[{"role":"aut","display":"Kraack, Jan Philip","roleDisplay":"VerfasserIn","given":"Jan Philip","family":"Kraack"},{"display":"Buckup, Tiago","roleDisplay":"VerfasserIn","role":"aut","family":"Buckup","given":"Tiago"},{"display":"Motzkus, Marcus","roleDisplay":"VerfasserIn","role":"aut","family":"Motzkus","given":"Marcus"}],"title":[{"title_sort":"Coherent high-frequency vibrational dynamics in the excited electronic state of all-trans retinal derivatives","title":"Coherent high-frequency vibrational dynamics in the excited electronic state of all-trans retinal derivatives"}],"physDesc":[{"extent":"5 S."}],"relHost":[{"title":[{"title_sort":"journal of physical chemistry letters","title":"The journal of physical chemistry letters"}],"pubHistory":["1.2010 -"],"titleAlt":[{"title":"JPCLett"}],"part":{"text":"4(2013), 3, Seite 383-387","volume":"4","extent":"5","year":"2013","issue":"3","pages":"383-387"},"disp":"Coherent high-frequency vibrational dynamics in the excited electronic state of all-trans retinal derivativesThe journal of physical chemistry letters","note":["Gesehen am 02.01.2013"],"type":{"media":"Online-Ressource","bibl":"periodical"},"language":["eng"],"recId":"612168581","origin":[{"dateIssuedDisp":"2010-","dateIssuedKey":"2010","publisher":"ACS","publisherPlace":"Washington, DC"}],"id":{"zdb":["2522838-9"],"eki":["612168581"],"issn":["1948-7185"]},"name":{"displayForm":["American Chemical Society"]},"physDesc":[{"extent":"Online-Ressource"}]}],"name":{"displayForm":["Jan Philip Kraack, Tiago Buckup, and Marcus Motzkus"]},"origin":[{"dateIssuedKey":"2013","dateIssuedDisp":"January 10, 2013"}],"id":{"doi":["10.1021/jz302001m"],"eki":["175258371X"]}} | ||
| SRT | |a KRAACKJANPCOHERENTHI1020 | ||