Nonlinear absorption in interacting Rydberg electromagnetically-induced-transparency spectra on two-photon resonance
We experimentally investigate the nonlinear transmission spectrum of coherent light fields propagating through a Rydberg EIT medium with strong atomic interactions. In contrast to previous investigations, which have largely focused on resonant control fields, we explore here the full two-dimensional...
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| Hauptverfasser: | , , , , , , , , |
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| Dokumenttyp: | Article (Journal) |
| Sprache: | Englisch |
| Veröffentlicht: |
24 June 2021
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| In: |
Physical review
Year: 2021, Jahrgang: 103, Heft: 6, Pages: 1-11 |
| ISSN: | 2469-9934 |
| DOI: | 10.1103/PhysRevA.103.063710 |
| Online-Zugang: | Verlag, lizenzpflichtig, Volltext: https://doi.org/10.1103/PhysRevA.103.063710 Verlag, lizenzpflichtig, Volltext: https://link.aps.org/doi/10.1103/PhysRevA.103.063710 
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| Verfasserangaben: | Annika Tebben, Clément Hainaut, Andre Salzinger, Sebastian Geier, Titus Franz, Thomas Pohl, Martin Gärttner, Gerhard Zürn, and Matthias Weidemüller |
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| 245 | 1 | 0 | |a Nonlinear absorption in interacting Rydberg electromagnetically-induced-transparency spectra on two-photon resonance |c Annika Tebben, Clément Hainaut, Andre Salzinger, Sebastian Geier, Titus Franz, Thomas Pohl, Martin Gärttner, Gerhard Zürn, and Matthias Weidemüller |
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| 520 | |a We experimentally investigate the nonlinear transmission spectrum of coherent light fields propagating through a Rydberg EIT medium with strong atomic interactions. In contrast to previous investigations, which have largely focused on resonant control fields, we explore here the full two-dimensional spectral response of the Rydberg gas. Our measurements confirm previously observed spectral features for a vanishing control-field detuning, but also reveal significant differences on two-photon resonance. In particular, we find qualitative deficiencies of mean-field models and rate-equation simulations as well as a third-order nonlinear susceptibility that accounts for pairwise interaction effects at low probe-field intensities in describing the nonlinear probe-field response under EIT conditions. Our results suggest that a more complete understanding of Rydberg EIT and emerging photon interactions requires to go beyond existing simplified models as well as few-photon theories. | ||
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