Quasi-1D XY antiferromagnet Sr2Ni(SeO3)2Cl2 at Sakai-Takahashi phase diagram
Uniform quasi-one-dimensional integer spin compounds are of interest as a potential realization of the Haldane conjecture of a gapped spin liquid. This phase, however, has to compete with magnetic anisotropy and long-range ordered phases, the implementation of which depends on the ratio of interchai...
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| Hauptverfasser: | , , , , , , , , , |
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| Dokumenttyp: | Article (Journal) |
| Sprache: | Englisch |
| Veröffentlicht: |
22 July 2021
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| In: |
Scientific reports
Year: 2021, Jahrgang: 11, Pages: 1-8 |
| ISSN: | 2045-2322 |
| DOI: | 10.1038/s41598-021-94390-3 |
| Online-Zugang: | Verlag, lizenzpflichtig, Volltext: https://doi.org/10.1038/s41598-021-94390-3 Verlag, lizenzpflichtig, Volltext: https://www.nature.com/articles/s41598-021-94390-3 
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| Verfasserangaben: | E.S. Kozlyakova, A.V. Moskin, P.S. Berdonosov, V.V. Gapontsev, S.V. Streltsov, M. Uhlarz, S. Spachmann, A. ElGhandour, R. Klingeler & A.N. Vasiliev |
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| 245 | 1 | 0 | |a Quasi-1D XY antiferromagnet Sr2Ni(SeO3)2Cl2 at Sakai-Takahashi phase diagram |c E.S. Kozlyakova, A.V. Moskin, P.S. Berdonosov, V.V. Gapontsev, S.V. Streltsov, M. Uhlarz, S. Spachmann, A. ElGhandour, R. Klingeler & A.N. Vasiliev |
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| 520 | |a Uniform quasi-one-dimensional integer spin compounds are of interest as a potential realization of the Haldane conjecture of a gapped spin liquid. This phase, however, has to compete with magnetic anisotropy and long-range ordered phases, the implementation of which depends on the ratio of interchain J′ and intrachain J exchange interactions and both uniaxial D and rhombic E single-ion anisotropies. Strontium nickel selenite chloride, Sr2Ni(SeO3)2Cl2, is a spin-1 chain system which passes through a correlations regime at Tmax ~ 12 K to long-range order at TN = 6 K. Under external magnetic field it experiences the sequence of spin-flop at Bc1 = 9.0 T and spin-flip transitions Bc2 = 23.7 T prior to full saturation at Bsat = 31.0 T. Density functional theory provides values of the main exchange interactions and uniaxial anisotropy which corroborate the experimental findings. The values of J′/J = 0.083 and D/J = 0.357 place this compound into a hitherto unoccupied sector of the Sakai-Takahashi phase diagram. | ||
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