Lorentz meets Fano in spectral line shapes: a universal phase and its laser control
Symmetric Lorentzian and asymmetric Fano line shapes are fundamental spectroscopic signatures that quantify the structural and dynamical properties of nuclei, atoms, molecules, and solids. This study introduces a universal temporal-phase formalism, mapping the Fano asymmetry parameter q to a phase φ...
Gespeichert in:
| Hauptverfasser: | , , , , , , , , |
|---|---|
| Dokumenttyp: | Article (Journal) |
| Sprache: | Englisch |
| Veröffentlicht: |
10 May 2013
|
| In: |
Science
Year: 2013, Jahrgang: 340, Heft: 6133, Pages: 716-720 |
| ISSN: | 1095-9203 |
| DOI: | 10.1126/science.1234407 |
| Online-Zugang: | Verlag, lizenzpflichtig, Volltext: https://doi.org/10.1126/science.1234407 Verlag, lizenzpflichtig, Volltext: https://www.science.org/doi/10.1126/science.1234407 
|
| Verfasserangaben: | Christian Ott, Andreas Kaldun, Philipp Raith, Kristina Meyer, Martin Laux, Jörg Evers, Christoph H. Keitel, Chris H. Greene, Thomas Pfeifer |
MARC
| LEADER | 00000caa a2200000 c 4500 | ||
|---|---|---|---|
| 001 | 1780847831 | ||
| 003 | DE-627 | ||
| 005 | 20220820091827.0 | ||
| 007 | cr uuu---uuuuu | ||
| 008 | 211209s2013 xx |||||o 00| ||eng c | ||
| 024 | 7 | |a 10.1126/science.1234407 |2 doi | |
| 035 | |a (DE-627)1780847831 | ||
| 035 | |a (DE-599)KXP1780847831 | ||
| 035 | |a (OCoLC)1341434467 | ||
| 040 | |a DE-627 |b ger |c DE-627 |e rda | ||
| 041 | |a eng | ||
| 084 | |a 29 |2 sdnb | ||
| 100 | 1 | |a Ott, Christian |e VerfasserIn |0 (DE-588)1024756459 |0 (DE-627)720459516 |0 (DE-576)369446283 |4 aut | |
| 245 | 1 | 0 | |a Lorentz meets Fano in spectral line shapes |b a universal phase and its laser control |c Christian Ott, Andreas Kaldun, Philipp Raith, Kristina Meyer, Martin Laux, Jörg Evers, Christoph H. Keitel, Chris H. Greene, Thomas Pfeifer |
| 264 | 1 | |c 10 May 2013 | |
| 300 | |a 5 | ||
| 336 | |a Text |b txt |2 rdacontent | ||
| 337 | |a Computermedien |b c |2 rdamedia | ||
| 338 | |a Online-Ressource |b cr |2 rdacarrier | ||
| 500 | |a Gesehen am 09.12.2021 | ||
| 520 | |a Symmetric Lorentzian and asymmetric Fano line shapes are fundamental spectroscopic signatures that quantify the structural and dynamical properties of nuclei, atoms, molecules, and solids. This study introduces a universal temporal-phase formalism, mapping the Fano asymmetry parameter q to a phase φof the time-dependent dipole response function. The formalism is confirmed experimentally by laser-transforming Fano absorption lines of autoionizing helium into Lorentzian lines after attosecond-pulsed excitation. We also demonstrate the inverse, the transformation of a naturally Lorentzian line into a Fano profile. A further application of this formalism uses quantum-phase control to amplify extreme-ultraviolet light resonantly interacting with He atoms. The quantum phase of excited states and its response to interactions can thus be extracted from line-shape analysis, with applications in many branches of spectroscopy. | ||
| 700 | 1 | |a Kaldun, Andreas |e VerfasserIn |0 (DE-588)1051965780 |0 (DE-627)787216356 |0 (DE-576)407627537 |4 aut | |
| 700 | 1 | |a Raith, Philipp Nils |e VerfasserIn |0 (DE-588)1028597304 |0 (DE-627)731305973 |0 (DE-576)376089202 |4 aut | |
| 700 | 1 | |a Meyer, Kristina |e VerfasserIn |0 (DE-588)1062728564 |0 (DE-627)80681599X |0 (DE-576)420111131 |4 aut | |
| 700 | 1 | |a Laux, Martin |d 1985- |e VerfasserIn |0 (DE-588)14301921X |0 (DE-627)641850271 |0 (DE-576)33463301X |4 aut | |
| 700 | 1 | |a Evers, Jörg |d 1976- |e VerfasserIn |0 (DE-588)1073947106 |0 (DE-627)830052321 |0 (DE-576)435446827 |4 aut | |
| 700 | 1 | |a Keitel, Christoph H. |d 1965- |e VerfasserIn |0 (DE-588)1012769488 |0 (DE-627)699763630 |0 (DE-576)170520188 |4 aut | |
| 700 | 1 | |a Greene, Chris H. |e VerfasserIn |4 aut | |
| 700 | 1 | |a Pfeifer, Thomas |d 1977- |e VerfasserIn |0 (DE-588)130276197 |0 (DE-627)497357836 |0 (DE-576)298101165 |4 aut | |
| 773 | 0 | 8 | |i Enthalten in |t Science |d Washington, DC : American Association for the Advancement of Science, 1880 |g 340(2013), 6133, Seite 716-720 |h Online-Ressource |w (DE-627)341342882 |w (DE-600)2066996-3 |w (DE-576)099426773 |x 1095-9203 |7 nnas |a Lorentz meets Fano in spectral line shapes a universal phase and its laser control |
| 773 | 1 | 8 | |g volume:340 |g year:2013 |g number:6133 |g pages:716-720 |g extent:5 |a Lorentz meets Fano in spectral line shapes a universal phase and its laser control |
| 856 | 4 | 0 | |u https://doi.org/10.1126/science.1234407 |x Verlag |x Resolving-System |z lizenzpflichtig |3 Volltext |
| 856 | 4 | 0 | |u https://www.science.org/doi/10.1126/science.1234407 |x Verlag |z lizenzpflichtig |3 Volltext |
| 951 | |a AR | ||
| 992 | |a 20211209 | ||
| 993 | |a Article | ||
| 994 | |a 2013 | ||
| 998 | |g 130276197 |a Pfeifer, Thomas |m 130276197:Pfeifer, Thomas |d 130000 |e 130000PP130276197 |k 0/130000/ |p 9 |y j | ||
| 998 | |g 1012769488 |a Keitel, Christoph H. |m 1012769488:Keitel, Christoph H. |d 130000 |e 130000PK1012769488 |k 0/130000/ |p 7 | ||
| 998 | |g 1073947106 |a Evers, Jörg |m 1073947106:Evers, Jörg |d 130000 |e 130000PE1073947106 |k 0/130000/ |p 6 | ||
| 998 | |g 1062728564 |a Meyer, Kristina |m 1062728564:Meyer, Kristina |d 130000 |e 130000PM1062728564 |k 0/130000/ |p 4 | ||
| 998 | |g 1051965780 |a Kaldun, Andreas |m 1051965780:Kaldun, Andreas |d 130000 |e 130000PK1051965780 |k 0/130000/ |p 2 | ||
| 998 | |g 1024756459 |a Ott, Christian |m 1024756459:Ott, Christian |d 130000 |e 130000PO1024756459 |k 0/130000/ |p 1 |x j | ||
| 999 | |a KXP-PPN1780847831 |e 4017891586 | ||
| BIB | |a Y | ||
| SER | |a journal | ||
| JSO | |a {"physDesc":[{"extent":"5 S."}],"id":{"doi":["10.1126/science.1234407"],"eki":["1780847831"]},"person":[{"family":"Ott","display":"Ott, Christian","given":"Christian","role":"aut"},{"family":"Kaldun","role":"aut","given":"Andreas","display":"Kaldun, Andreas"},{"family":"Raith","role":"aut","given":"Philipp Nils","display":"Raith, Philipp Nils"},{"family":"Meyer","given":"Kristina","display":"Meyer, Kristina","role":"aut"},{"family":"Laux","display":"Laux, Martin","given":"Martin","role":"aut"},{"role":"aut","given":"Jörg","display":"Evers, Jörg","family":"Evers"},{"role":"aut","given":"Christoph H.","display":"Keitel, Christoph H.","family":"Keitel"},{"family":"Greene","display":"Greene, Chris H.","given":"Chris H.","role":"aut"},{"role":"aut","display":"Pfeifer, Thomas","given":"Thomas","family":"Pfeifer"}],"title":[{"title_sort":"Lorentz meets Fano in spectral line shapes","subtitle":"a universal phase and its laser control","title":"Lorentz meets Fano in spectral line shapes"}],"name":{"displayForm":["Christian Ott, Andreas Kaldun, Philipp Raith, Kristina Meyer, Martin Laux, Jörg Evers, Christoph H. Keitel, Chris H. Greene, Thomas Pfeifer"]},"language":["eng"],"type":{"media":"Online-Ressource","bibl":"article-journal"},"relHost":[{"titleAlt":[{"title":"Science / Magazine"},{"title":"Science classic"},{"title":"Science classic archiv 1880 - 1996"},{"title":"Science magazine"}],"corporate":[{"display":"American Association for the Advancement of Science","role":"isb"}],"part":{"year":"2013","pages":"716-720","text":"340(2013), 6133, Seite 716-720","volume":"340","extent":"5","issue":"6133"},"title":[{"title":"Science","title_sort":"Science"}],"disp":"Lorentz meets Fano in spectral line shapes a universal phase and its laser controlScience","physDesc":[{"extent":"Online-Ressource"}],"type":{"bibl":"periodical","media":"Online-Ressource"},"recId":"341342882","origin":[{"publisherPlace":"Washington, DC","publisher":"American Association for the Advancement of Science","dateIssuedDisp":"1880-","dateIssuedKey":"1880"}],"note":["Gesehen am 14.07.2023"],"pubHistory":["1.1880 - 3.1882; 1.1883 - 23.1894; N.S. 1.1895 -"],"id":{"issn":["1095-9203"],"zdb":["2066996-3"],"eki":["341342882"]},"language":["eng"],"name":{"displayForm":["AAAS"]}}],"recId":"1780847831","note":["Gesehen am 09.12.2021"],"origin":[{"dateIssuedDisp":"10 May 2013","dateIssuedKey":"2013"}]} | ||
| SRT | |a OTTCHRISTILORENTZMEE1020 | ||