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Vibrationally resolved decay width of interatomic Coulombic decay in HeNe

We investigate the ionization of HeNe from below the He 1s3p excitation to the He ionization threshold. We observe HeNe+ ions with an enhancement by more than a factor of 60 when the He side couples resonantly to the radiation field. These ions are an experimental proof of a two-center resonant phot...

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Main Authors: Trinter, Florian (Author) , Williams, J. B. (Author) , Weller, M. (Author) , Waitz, M. (Author) , Pitzer, M. (Author) , Voigtsberger, J. (Author) , Schober, C. (Author) , Kastirke, G. (Author) , Müller, C. (Author) , Goihl, C. (Author) , Burzynski, P. (Author) , Wiegandt, F. (Author) , Wallauer, R. (Author) , Kalinin, A. (Author) , Schmidt, L. Ph. H. (Author) , Schöffler, M. S. (Author) , Chiang, Ying-Chih (Author) , Gokhberg, Kirill (Author) , Jahnke, T. (Author) , Dörner, R. (Author)
Format: Article (Journal)
Language:English
Published: 4 December 2013
In: Physical review letters
Year: 2013, Volume: 111, Issue: 23, Pages: 1-5
ISSN:1079-7114
DOI:10.1103/PhysRevLett.111.233004
Online Access:Verlag, lizenzpflichtig, Volltext: https://doi.org/10.1103/PhysRevLett.111.233004
Verlag, lizenzpflichtig, Volltext: https://link.aps.org/doi/10.1103/PhysRevLett.111.233004
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Author Notes:F. Trinter, J.B. Williams, M. Weller, M. Waitz, M. Pitzer, J. Voigtsberger, C. Schober, G. Kastirke, C. Müller, C. Goihl, P. Burzynski, F. Wiegandt, R. Wallauer, A. Kalinin, L.Ph.H. Schmidt, M.S. Schöffler, Y.-C. Chiang, K. Gokhberg, T. Jahnke, and R. Dörner

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520 |a We investigate the ionization of HeNe from below the He 1s3p excitation to the He ionization threshold. We observe HeNe+ ions with an enhancement by more than a factor of 60 when the He side couples resonantly to the radiation field. These ions are an experimental proof of a two-center resonant photoionization mechanism predicted by Najjari et al. [Phys. Rev. Lett. 105, 153002 (2010)]. Furthermore, our data provide electronic and vibrational state resolved decay widths of interatomic Coulombic decay in HeNe dimers. We find that the interatomic Coulombic decay lifetime strongly increases with increasing vibrational state. 
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