Strong effects of uniaxial pressure and short-range correlations in Cr2Ge2Te6

Cr2Ge2Te6 is a quasi-two-dimensional semiconducting van der Waals ferromagnet down to the bilayer with great potential for technological applications. Engineering the critical temperature to achieve room-temperature applications is one of the critical next steps on this path. Here, we report high-re...

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Hauptverfasser: Spachmann, Sven (VerfasserIn) , Elghandour, Ahmed (VerfasserIn) , Selter, Sebastian (VerfasserIn) , Büchner, Bernd (VerfasserIn) , Aswartham, Saicharan (VerfasserIn) , Klingeler, Rüdiger (VerfasserIn)
Dokumenttyp: Article (Journal) Editorial
Sprache:Englisch
Veröffentlicht: 20 May 2022
In: Physical review research
Year: 2022, Jahrgang: 4, Heft: 2, Pages: 1-7
ISSN:2643-1564
DOI:10.1103/PhysRevResearch.4.L022040
Online-Zugang:Verlag, lizenzpflichtig, Volltext: https://doi.org/10.1103/PhysRevResearch.4.L022040
Verlag, lizenzpflichtig, Volltext: https://link.aps.org/doi/10.1103/PhysRevResearch.4.L022040
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Verfasserangaben:S. Spachmann, A. Elghandour, S. Selter, B. Büchner, S. Aswartham, and R. Klingeler

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520 |a Cr2Ge2Te6 is a quasi-two-dimensional semiconducting van der Waals ferromagnet down to the bilayer with great potential for technological applications. Engineering the critical temperature to achieve room-temperature applications is one of the critical next steps on this path. Here, we report high-resolution capacitance dilatometry studies on Cr2Ge2Te6 single crystals which directly prove significant magnetoelastic coupling and provide quantitative values of the large uniaxial pressure effects on long-range magnetic order (∂TC/∂pc=24.7 K/GPa and ∂TC/∂pab=−15.6 K/GPa) derived from thermodynamic relations. Moderate in-plane strain is thus sufficient to strongly enhance ferromagnetism in Cr2Ge2Te6 up to room temperature. Moreover, unambiguous signs of short-range magnetic order up to 200 K are found. 
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