Tailored solution-based N-heterotriangulene thin films: unravelling the self-assembly
The ability of a series of bridged triarylamines, so-called N-heterotriangulenes, to form multilayer-type 2D-extended films via a solution-based processing method was examined using complementary microscopic techniques. We found that the long-range order, crystallinity, and layer thickness decisivel...
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| Hauptverfasser: | , , , , , , , , , , , |
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| Dokumenttyp: | Article (Journal) |
| Sprache: | Englisch |
| Veröffentlicht: |
01 April 2021
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| In: |
ChemPhysChem
Year: 2021, Jahrgang: 22, Heft: 11, Pages: 1079-1087 |
| ISSN: | 1439-7641 |
| DOI: | 10.1002/cphc.202100164 |
| Online-Zugang: | Verlag, lizenzpflichtig, Volltext: https://doi.org/10.1002/cphc.202100164 Verlag, lizenzpflichtig, Volltext: https://onlinelibrary.wiley.com/doi/abs/10.1002/cphc.202100164 
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| Verfasserangaben: | Tim Hawly, Fabian Streller, Manuel Johnson, Sandra Miguez-Lago, Natalie Hammer, Frank Hampel, Dustin Vivod, Dirk Zahn, Milan Kivala, Robert Branscheid, Erdmann Spiecker, and Rainer H. Fink |
MARC
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| 520 | |a The ability of a series of bridged triarylamines, so-called N-heterotriangulenes, to form multilayer-type 2D-extended films via a solution-based processing method was examined using complementary microscopic techniques. We found that the long-range order, crystallinity, and layer thickness decisively depend on the nature of the substituents attached to the polycyclic backbone. Owing to their flat core unit, compounds exhibiting a carbonyl unit at the bridge position provide a superior building block as compared to thioketone-bridged derivatives. In addition, nature and length of the peripheral substituents affect the orientation of the aromatic core unit within highly crystalline films. Hence, our results stress the significance of a suitable molecular framework and provide deeper understanding of structure formation in 2D-confined surroundings for such compounds. | ||
| 650 | 4 | |a 2D nanomaterials | |
| 650 | 4 | |a bridged triarylamines | |
| 650 | 4 | |a organic electronics | |
| 650 | 4 | |a organic semiconductors | |
| 650 | 4 | |a self-assembly | |
| 700 | 1 | |a Streller, Fabian |e VerfasserIn |4 aut | |
| 700 | 1 | |a Johnson, Manuel |e VerfasserIn |4 aut | |
| 700 | 1 | |a Miguez-Lago, Sandra |e VerfasserIn |4 aut | |
| 700 | 1 | |a Hammer, Natalie |e VerfasserIn |4 aut | |
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| 700 | 1 | |a Vivod, Dustin |e VerfasserIn |4 aut | |
| 700 | 1 | |a Zahn, Dirk |e VerfasserIn |4 aut | |
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| 700 | 1 | |a Branscheid, Robert |e VerfasserIn |4 aut | |
| 700 | 1 | |a Spiecker, Erdmann |e VerfasserIn |4 aut | |
| 700 | 1 | |a Fink, Rainer H. |e VerfasserIn |4 aut | |
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