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Saturation field of frustrated chain cuprates: broad regions of predominant interchain coupling

A thermodynamic method to extract the interchain coupling (IC) of spatially anisotropic 2D or 3D spin-1/2 systems from their empirical saturation field Hs (T=0) is proposed. Using modern theoretical methods we study how Hs is affected by an antiferromagnetic (AFM) IC between frustrated chains descri...

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Main Authors: Nishimoto, Satoshi (Author) , Drechsler, S.-L. (Author) , Kuzian, R. O. (Author) , van den Brink, J. (Author) , Richter, J. (Author) , Lorenz, W. E. A. (Author) , Skourski, Y. (Author) , Klingeler, Rüdiger (Author) , Büchner, B. (Author)
Format: Article (Journal)
Language:English
Published: 22 August 2011
In: Physical review letters
Year: 2011, Volume: 107, Issue: 9, Pages: 1-4
ISSN:1079-7114
DOI:10.1103/PhysRevLett.107.097201
Online Access:Verlag, lizenzpflichtig, Volltext: https://doi.org/10.1103/PhysRevLett.107.097201
Verlag, lizenzpflichtig, Volltext: https://link.aps.org/doi/10.1103/PhysRevLett.107.097201
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Author Notes:S. Nishimoto, S.-L. Drechsler, R.O. Kuzian, J. van den Brink, J. Richter, W.E.A. Lorenz, Y. Skourski, R. Klingeler, and B. Büchner

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520 |a A thermodynamic method to extract the interchain coupling (IC) of spatially anisotropic 2D or 3D spin-1/2 systems from their empirical saturation field Hs (T=0) is proposed. Using modern theoretical methods we study how Hs is affected by an antiferromagnetic (AFM) IC between frustrated chains described in the J1−J2-spin model with ferromagnetic 1st and AFM 2nd neighbor in-chain exchange. A complex 3D-phase diagram has been found. For Li2CuO2 and Ca2Y2Cu5O10, we show that Hs is solely determined by the IC and predict Hs≈61 T for the latter. With Hs≈55 T from magnetization data one reads out a weak IC for Li2CuO2 close to that obtained from inelastic neutron scattering. 
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