An improved hydrolytically-stable Bis-Triazinyl-Pyridine (BTP) for selective actinide extraction
Bis-2,6-(5,6,7,8-tetrahydro-5,9,9-trimethyl-5,8-methano-1,2,4-benzotriazin-3-yl)pyridine (CA-BTP) is presented as a novel optimized extracting agent for the separation of americium(III) and curium(III) from lanthanides(III). CA-BTP is synthesized and studied concerning its extraction properties unde...
Gespeichert in:
| Hauptverfasser: | , , , |
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| Dokumenttyp: | Article (Journal) |
| Sprache: | Englisch |
| Veröffentlicht: |
30 Mar 2011
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| In: |
Solvent extraction and ion exchange
Year: 2011, Jahrgang: 29, Heft: 2, Pages: 213-229 |
| ISSN: | 1532-2262 |
| DOI: | 10.1080/07366299.2011.539129 |
| Online-Zugang: | Verlag, lizenzpflichtig, Volltext: https://doi.org/10.1080/07366299.2011.539129
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| Verfasserangaben: | Sascha Trumm, Andreas Geist, Petra J. Panak & Thomas Fanghänel |
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| 520 | |a Bis-2,6-(5,6,7,8-tetrahydro-5,9,9-trimethyl-5,8-methano-1,2,4-benzotriazin-3-yl)pyridine (CA-BTP) is presented as a novel optimized extracting agent for the separation of americium(III) and curium(III) from lanthanides(III). CA-BTP is synthesized and studied concerning its extraction properties under conditions relevant to the SANEX process. It is demonstrated that CA-BTP is the first relevant molecule to show both high stability towards highly-acidic process solutions and satisfactory extraction kinetics. Its high solubility in 1-octanol adds to CA-BTP's favorable properties. Furthermore, CA-BTP is synthesized from a commercially available and moderately priced precursor molecule, reducing extracting-agent production costs. | ||
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