Revealing molecular orbital gating by transition voltage spectroscopy
Recently, Song et al. [Nature 462, 1039 (2009)] employed transition voltage spectroscopy to demonstrate that the energy εH of the highest occupied molecular orbital (HOMO) of single-molecule transistors can be controlled by a gate potential VG. To demonstrate the linear dependence εH−VG, the experim...
Gespeichert in:
| 1. Verfasser: | |
|---|---|
| Dokumenttyp: | Article (Journal) |
| Sprache: | Englisch |
| Veröffentlicht: |
11 August 2010
|
| In: |
Chemical physics
Year: 2010, Jahrgang: 377, Heft: 1, Pages: 15-20 |
| DOI: | 10.1016/j.chemphys.2010.08.009 |
| Online-Zugang: | Verlag, lizenzpflichtig, Volltext: https://doi.org/10.1016/j.chemphys.2010.08.009 Verlag, lizenzpflichtig, Volltext: https://www.sciencedirect.com/science/article/pii/S0301010410003794 
|
| Verfasserangaben: | Ioan Bâldea |
MARC
| LEADER | 00000caa a2200000 c 4500 | ||
|---|---|---|---|
| 001 | 1823593119 | ||
| 003 | DE-627 | ||
| 005 | 20230710163312.0 | ||
| 007 | cr uuu---uuuuu | ||
| 008 | 221125s2010 xx |||||o 00| ||eng c | ||
| 024 | 7 | |a 10.1016/j.chemphys.2010.08.009 |2 doi | |
| 035 | |a (DE-627)1823593119 | ||
| 035 | |a (DE-599)KXP1823593119 | ||
| 035 | |a (OCoLC)1389822575 | ||
| 040 | |a DE-627 |b ger |c DE-627 |e rda | ||
| 041 | |a eng | ||
| 084 | |a 29 |2 sdnb | ||
| 100 | 1 | |a Bâldea, Ioan |e VerfasserIn |0 (DE-588)1049572033 |0 (DE-627)782333303 |0 (DE-576)403568498 |4 aut | |
| 245 | 1 | 0 | |a Revealing molecular orbital gating by transition voltage spectroscopy |c Ioan Bâldea |
| 264 | 1 | |c 11 August 2010 | |
| 300 | |a 6 | ||
| 336 | |a Text |b txt |2 rdacontent | ||
| 337 | |a Computermedien |b c |2 rdamedia | ||
| 338 | |a Online-Ressource |b cr |2 rdacarrier | ||
| 500 | |a Gesehen am 25.11.2022 | ||
| 520 | |a Recently, Song et al. [Nature 462, 1039 (2009)] employed transition voltage spectroscopy to demonstrate that the energy εH of the highest occupied molecular orbital (HOMO) of single-molecule transistors can be controlled by a gate potential VG. To demonstrate the linear dependence εH−VG, the experimental data have been interpreted by modeling the molecule as an energy barrier spanning the spatial source-drain region of molecular junctions. Since, as shown in this work, that crude model cannot quantitatively describe the measured I-V-characteristics, it is important to get further support for the linear dependence of εH on VG. The results presented here, which have been obtained within a model of a point-like molecule, confirm this linear dependence. Because the two models rely upon complementary descriptions, the present results indicate that the interpretation of the experimental results as evidence for a gate controlled HOMO is sufficiently general. | ||
| 650 | 4 | |a Fowler-Nordheim transition | |
| 650 | 4 | |a Molecular electronics | |
| 650 | 4 | |a Molecular orbital gating | |
| 650 | 4 | |a Quantum transport | |
| 650 | 4 | |a Single-molecule transistors | |
| 650 | 4 | |a Transition voltage spectroscopy | |
| 773 | 0 | 8 | |i Enthalten in |t Chemical physics |d Amsterdam [u.a.] : Elsevier Science, 1973 |g 377(2010), 1, Seite 15-20 |h Online-Ressource |w (DE-627)306717867 |w (DE-600)1501546-4 |w (DE-576)09408551X |7 nnas |a Revealing molecular orbital gating by transition voltage spectroscopy |
| 773 | 1 | 8 | |g volume:377 |g year:2010 |g number:1 |g pages:15-20 |g extent:6 |a Revealing molecular orbital gating by transition voltage spectroscopy |
| 856 | 4 | 0 | |u https://doi.org/10.1016/j.chemphys.2010.08.009 |x Verlag |x Resolving-System |z lizenzpflichtig |3 Volltext |
| 856 | 4 | 0 | |u https://www.sciencedirect.com/science/article/pii/S0301010410003794 |x Verlag |z lizenzpflichtig |3 Volltext |
| 951 | |a AR | ||
| 992 | |a 20221125 | ||
| 993 | |a Article | ||
| 994 | |a 2010 | ||
| 998 | |g 1049572033 |a Bâldea, Ioan |m 1049572033:Bâldea, Ioan |d 120000 |d 120300 |e 120000PB1049572033 |e 120300PB1049572033 |k 0/120000/ |k 1/120000/120300/ |p 1 |x j |y j | ||
| 999 | |a KXP-PPN1823593119 |e 4219462090 | ||
| BIB | |a Y | ||
| SER | |a journal | ||
| JSO | |a {"physDesc":[{"extent":"6 S."}],"relHost":[{"physDesc":[{"extent":"Online-Ressource"}],"id":{"zdb":["1501546-4"],"eki":["306717867"]},"origin":[{"dateIssuedKey":"1973","publisher":"Elsevier Science","dateIssuedDisp":"1973-","publisherPlace":"Amsterdam [u.a.]"}],"language":["eng"],"recId":"306717867","type":{"bibl":"periodical","media":"Online-Ressource"},"disp":"Revealing molecular orbital gating by transition voltage spectroscopyChemical physics","note":["Gesehen am 14.02.06"],"part":{"extent":"6","text":"377(2010), 1, Seite 15-20","volume":"377","pages":"15-20","issue":"1","year":"2010"},"pubHistory":["1.1973 - 389.2011; Vol. 390.2011 -"],"title":[{"title_sort":"Chemical physics","subtitle":"a journal devoted to experimental and theoretical research involving problems of both a chemical and physical nature","title":"Chemical physics"}]}],"origin":[{"dateIssuedDisp":"11 August 2010","dateIssuedKey":"2010"}],"id":{"doi":["10.1016/j.chemphys.2010.08.009"],"eki":["1823593119"]},"name":{"displayForm":["Ioan Bâldea"]},"note":["Gesehen am 25.11.2022"],"type":{"bibl":"article-journal","media":"Online-Ressource"},"recId":"1823593119","language":["eng"],"title":[{"title":"Revealing molecular orbital gating by transition voltage spectroscopy","title_sort":"Revealing molecular orbital gating by transition voltage spectroscopy"}],"person":[{"role":"aut","roleDisplay":"VerfasserIn","display":"Bâldea, Ioan","given":"Ioan","family":"Bâldea"}]} | ||
| SRT | |a BALDEAIOANREVEALINGM1120 | ||