Electron-beam lithography of cinnamate polythiophene films: conductive nanorods for electronic applications
We report the electron-beam induced crosslinking of cinnamate-substituted polythiophene proceeding via excited state [2+2]-cycloaddition. Network formation in thin films is evidenced by infrared spectroscopy and film retention experiments. For the polymer studied herin, the electron-stimulated proce...
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| Hauptverfasser: | , , , , , , , , , , |
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| Dokumenttyp: | Article (Journal) |
| Sprache: | Englisch |
| Veröffentlicht: |
16 Jun 2022
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| In: |
Chemical science
Year: 2022, Jahrgang: 13, Heft: 26, Pages: 7880-7885 |
| ISSN: | 2041-6539 |
| DOI: | 10.1039/D2SC01867E |
| Online-Zugang: | Verlag, kostenfrei, Volltext: https://doi.org/10.1039/D2SC01867E Verlag, kostenfrei, Volltext: https://pubs.rsc.org/en/content/articlelanding/2022/sc/d2sc01867e 
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| Verfasserangaben: | N. Maximilian Bojanowski, Christian Huck, Lisa Veith, Karl-Philipp Strunk, Rainer Bäuerle, Christian Melzer, Jan Freudenberg, Irene Wacker, Rasmus R. Schröder, Petra Tegeder and Uwe H.F. Bunz |
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| 245 | 1 | 0 | |a Electron-beam lithography of cinnamate polythiophene films |b conductive nanorods for electronic applications |c N. Maximilian Bojanowski, Christian Huck, Lisa Veith, Karl-Philipp Strunk, Rainer Bäuerle, Christian Melzer, Jan Freudenberg, Irene Wacker, Rasmus R. Schröder, Petra Tegeder and Uwe H.F. Bunz |
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| 520 | |a We report the electron-beam induced crosslinking of cinnamate-substituted polythiophene proceeding via excited state [2+2]-cycloaddition. Network formation in thin films is evidenced by infrared spectroscopy and film retention experiments. For the polymer studied herin, the electron-stimulated process appears to be superior to photo (UV)-induced crosslinking as it leads to less degradation. Electron beam lithography (EBL) patterns cinnamate-substituted polythiophene thin films on the nanoscale with a resolution of around 100 nm. As a proof of concept, we fabricated nanoscale organic transistors using doped and cross-linked P3ZT as contact fingers in thin film transistors. | ||
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