Highly conductive and long-term stable films from liquid-phase exfoliated platinum diselenide
Liquid-phase exfoliation (LPE) has been introduced as a versatile and scalable production method for two-dimensional (2D) materials. This method yields dispersions that allow for the fabrication of printable and flexible electronic devices. However, the fabrication of uniform and homogeneous films f...
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| Hauptverfasser: | , , , , , , , , , , , , |
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| Dokumenttyp: | Article (Journal) |
| Sprache: | Englisch |
| Veröffentlicht: |
2023
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| In: |
Journal of materials chemistry. C, Materials for optical and electronic devices
Year: 2023, Jahrgang: 11, Heft: 2, Pages: 593-599 |
| ISSN: | 2050-7534 |
| DOI: | 10.1039/D2TC03889G |
| Online-Zugang: | Verlag, lizenzpflichtig, Volltext: https://doi.org/10.1039/D2TC03889G Verlag, lizenzpflichtig, Volltext: https://pubs.rsc.org/en/content/articlelanding/2023/tc/d2tc03889g 
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| Verfasserangaben: | Kangho Lee, Beata M. Szydłowska, Oliver Hartwig, Kevin Synnatschke, Bartlomiej Tywoniuk, Tomáš Hartman, Tijana Tomašević-Ilić, Cian P. Gabbett, Jonathan N. Coleman, Zdeněk Sofer, Marko Spasenović, Claudia Backes and Georg S. Duesberg |
MARC
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| 245 | 1 | 0 | |a Highly conductive and long-term stable films from liquid-phase exfoliated platinum diselenide |c Kangho Lee, Beata M. Szydłowska, Oliver Hartwig, Kevin Synnatschke, Bartlomiej Tywoniuk, Tomáš Hartman, Tijana Tomašević-Ilić, Cian P. Gabbett, Jonathan N. Coleman, Zdeněk Sofer, Marko Spasenović, Claudia Backes and Georg S. Duesberg |
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| 520 | |a Liquid-phase exfoliation (LPE) has been introduced as a versatile and scalable production method for two-dimensional (2D) materials. This method yields dispersions that allow for the fabrication of printable and flexible electronic devices. However, the fabrication of uniform and homogeneous films from LPE dispersions with a performance similar to that of bottom-up grown materials remains a challenge, as the film quality strongly influences the optical and electrical performance of devices. Furthermore, long-term stability remains a major challenge for all 2D material based applications. In this study, we report on highly conductive tiled network films made of platinum diselenide (PtSe2) flakes derived using a scalable LPE method. We characterized the homogeneous films in terms of morphology and electrical behavior. As an example of applicability, we produce a chemiresistive sensor structure with the PtSe2 films and show significant resistance changes upon periodic ammonia gas exposures, revealing a sub-0.1 part per million (ppm) detection limit (DL). More remarkably the devices are fully functional after 15 months, underlining the high stability of PtSe2 based devices. | ||
| 700 | 1 | |a Szydłowska, Beata Maria |e VerfasserIn |0 (DE-588)1188646524 |0 (DE-627)1667614665 |4 aut | |
| 700 | 1 | |a Hartwig, Oliver |e VerfasserIn |4 aut | |
| 700 | 1 | |a Synnatschke, Kevin |e VerfasserIn |4 aut | |
| 700 | 1 | |a Tywoniuk, Bartlomiej |e VerfasserIn |4 aut | |
| 700 | 1 | |a Hartman, Tomáš |e VerfasserIn |4 aut | |
| 700 | 1 | |a Tomašević-Ilić, Tijana |e VerfasserIn |4 aut | |
| 700 | 1 | |a Gabbett, Cian P. |e VerfasserIn |4 aut | |
| 700 | 1 | |a Coleman, Jonathan N. |e VerfasserIn |4 aut | |
| 700 | 1 | |a Sofer, Zdeněk |e VerfasserIn |4 aut | |
| 700 | 1 | |a Spasenović, Marko |e VerfasserIn |4 aut | |
| 700 | 1 | |a Backes, Claudia |d 1982- |e VerfasserIn |0 (DE-588)1019617233 |0 (DE-627)685502767 |0 (DE-576)358450535 |4 aut | |
| 700 | 1 | |a Duesberg, Georg S. |e VerfasserIn |4 aut | |
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