Interplay between structure and magnetism in Fe/Cu(1 0 0) upon temperature variation

Interleaved low-energy electron diffraction (LEED) and magneto-optical Kerr effect (MOKE) measurements were carried out for room-temperature epitaxially grown FCC-like Fe/Cu(1 0 0) in the temperature range of 120-400 K. The structure of the Fe film was found to be not only dependent on thickness, as...

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Hauptverfasser: Zharnikov, Michael (VerfasserIn) , Dittschar, A (VerfasserIn) , Kuch, W (VerfasserIn) , Schneider, C. M (VerfasserIn) , Kirschner, J (VerfasserIn)
Dokumenttyp: Article (Journal)
Sprache:Englisch
Veröffentlicht: 1 October 1997
In: Journal of magnetism and magnetic materials
Year: 1997, Jahrgang: 174, Heft: 1-2, Pages: 40-56
ISSN:1873-4766
DOI:10.1016/S0304-8853(97)00220-5
Online-Zugang:Verlag, lizenzpflichtig, Volltext: https://doi.org/10.1016/S0304-8853(97)00220-5
Verlag, lizenzpflichtig, Volltext: https://www.sciencedirect.com/science/article/pii/S0304885397002205
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Verfasserangaben:M. Zharnikov, A. Dittschar, W. Kuch, C.M. Schneider, J. Kirschner

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520 |a Interleaved low-energy electron diffraction (LEED) and magneto-optical Kerr effect (MOKE) measurements were carried out for room-temperature epitaxially grown FCC-like Fe/Cu(1 0 0) in the temperature range of 120-400 K. The structure of the Fe film was found to be not only dependent on thickness, as was believed previously, but also to be influenced by the temperature. Temperature-driven structural transitions were observed in the 4 and 4.5 ML films, this effect being more pronounced at 4 ML thickness. Whereas the whole 4 ML film assumes an FCC-like structure with a strong tetragonal expansion (FCT-like) at temperatures below 313 K, the bulk of the film relaxes into the ‘isotropic’ FCC-like structure and only the top layers remain expanded at temperatures above 333 K. Because only the FCT-like (expanded) Fe possesses ferromagnetic properties, the film becomes paramagnetic after heating above 333 K. This finding represents a new type of magnetic order-disorder transition and explains the lower value of the Curie temperature in the 4 ML Fe film as compared to 3 ML. In the 4.5 ML Fe film the similar correlation between the temperature-driven structural transition and an occurrence of the ferromagnetic long-range order was observed. Additionally, a pronounced difference in the energy positions of the characteristic maxima in the LEED I(E) curves for the (0 0) beam as well as a kinematic analysis of these curves imply a difference in the value of the tetragonal expansion for the entirely expanded FCC-like Fe film and the film expanded only in the topmost layers. 
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