Challenges and opportunities in 3D laser printing based on (1+1)-photon absorption
Most light-based 3D printing methods rely on optical or chemical nonlinearities to spatially confine the polymerization reaction. In 3D micro- and nanoprinting, this nonlinearity can be provided by two-photon absorption, which describes the simultaneous absorption of two photons. To achieve comparab...
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| Hauptverfasser: | , , , , , , , , , |
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| Dokumenttyp: | Article (Journal) |
| Sprache: | Englisch |
| Veröffentlicht: |
18 January 2023
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| In: |
ACS photonics
Year: 2023, Jahrgang: 10, Heft: 1, Pages: 24-33 |
| ISSN: | 2330-4022 |
| DOI: | 10.1021/acsphotonics.2c01632 |
| Online-Zugang: | Verlag, lizenzpflichtig, Volltext: https://doi.org/10.1021/acsphotonics.2c01632
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| Verfasserangaben: | Vincent Hahn, N. Maximilian Bojanowski, Pascal Rietz, Florian Feist, Mariana Kozlowska, Wolfgang Wenzel, Eva Blasco, Stefan Bräse, Christopher Barner-Kowollik, and Martin Wegener |
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| 520 | |a Most light-based 3D printing methods rely on optical or chemical nonlinearities to spatially confine the polymerization reaction. In 3D micro- and nanoprinting, this nonlinearity can be provided by two-photon absorption, which describes the simultaneous absorption of two photons. To achieve comparable absorption cross sections for two-photon as in one-photon absorption, short and intense laser pulses with intensities in the range of 1 TW/cm2 are typically required. Herein, we review three emerging excitation processes that provide a quadratic nonlinearity versus intensity without relying on two-photon absorption: upconversion luminescence, two-step absorption, and triplet-triplet annihilation. We term these “(1 + 1)-photon absorption”. Such processes allow for using continuous-wave lasers at much lower peak laser powers and at much lower cost than those typical for two-photon absorption. We review recent progress, describe current challenges, and outline future perspectives. | ||
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| 700 | 1 | |a Rietz, Pascal |e VerfasserIn |4 aut | |
| 700 | 1 | |a Feist, Florian |e VerfasserIn |4 aut | |
| 700 | 1 | |a Kozlowska, Mariana |e VerfasserIn |4 aut | |
| 700 | 1 | |a Wenzel, Wolfgang |e VerfasserIn |4 aut | |
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| 700 | 1 | |a Barner-Kowollik, Christopher |e VerfasserIn |4 aut | |
| 700 | 1 | |a Wegener, Martin |e VerfasserIn |4 aut | |
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