On the rising extra storage capacity of ultra-small Fe3O4 particles functionalized with HCS and their potential as high-performance anode material for electrochemical energy storage
We report a nanocomposite material exhibiting ultra-small Fe3O4 nanoparticles uniformly decorated on hollow carbon spheres (Fe3O4HCS). The unique hierarchically-structured material displays excellent electrochemical cycling performance that exceeds the theoretical bulk capacity of Fe3O4 when used as...
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| Main Authors: | , , , , , , , |
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| Format: | Article (Journal) |
| Language: | English |
| Published: |
9 March 2023
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| In: |
Electrochimica acta
Year: 2023, Volume: 448, Pages: 1-9 |
| ISSN: | 1873-3859 |
| DOI: | 10.1016/j.electacta.2023.142155 |
| Online Access: | Verlag, lizenzpflichtig, Volltext: https://doi.org/10.1016/j.electacta.2023.142155 Verlag, lizenzpflichtig, Volltext: https://www.sciencedirect.com/science/article/pii/S0013468623003390 
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| Author Notes: | Lennart Singer, Wojciech Kukułka, Elisa Thauer, Nico Gräßler, Andika Asyuda, Michael Zharnikov, Ewa Mijowska, Rüdiger Klingeler |
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| 520 | |a We report a nanocomposite material exhibiting ultra-small Fe3O4 nanoparticles uniformly decorated on hollow carbon spheres (Fe3O4HCS). The unique hierarchically-structured material displays excellent electrochemical cycling performance that exceeds the theoretical bulk capacity of Fe3O4 when used as an anode in lithium-ion batteries. In particular, it features increasing reversible capacity upon cycling yielding 1050 mAh g−1at 0.1 A g−1 in cycle 250. Comprehensive scanning and transmission electron microscopy images combined with detailed electrochemical analysis demonstrate that the outstanding electrochemical performance can be traced back to the formation and decomposition of a capacitative surface layer during dis/charging. | ||
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