Layered BiOI single crystals capable of detecting low dose rates of X-rays
Detecting low dose rates of X-rays is critical for making safer radiology instruments, but is limited by the absorber materials available. Here, we develop bismuth oxyiodide (BiOI) single crystals into effective X-ray detectors. BiOI features complex lattice dynamics, owing to the ionic character of...
Gespeichert in:
| Hauptverfasser: | , , , , , , , , , , , , , , , , , |
|---|---|
| Dokumenttyp: | Article (Journal) |
| Sprache: | Englisch |
| Veröffentlicht: |
28 April 2023
|
| In: |
Nature Communications
Year: 2023, Jahrgang: 14, Pages: 1-12 |
| ISSN: | 2041-1723 |
| DOI: | 10.1038/s41467-023-38008-4 |
| Online-Zugang: | Verlag, kostenfrei, Volltext: https://doi.org/10.1038/s41467-023-38008-4 Verlag, kostenfrei, Volltext: https://www.nature.com/articles/s41467-023-38008-4 
|
| Verfasserangaben: | Robert A. Jagt, Ivona Bravić, Lissa Eyre, Krzysztof Gałkowski, Joanna Borowiec, Kavya Reddy Dudipala, Michał Baranowski, Mateusz Dyksik, Tim W.J. van de Goor, Theo Kreouzis, Ming Xiao, Adrian Bevan, Paulina Płochocka, Samuel D. Stranks, Felix Deschler, Bartomeu Monserrat, Judith L. MacManus-Driscoll & Robert L.Z. Hoye |
MARC
| LEADER | 00000caa a2200000 c 4500 | ||
|---|---|---|---|
| 001 | 185765305X | ||
| 003 | DE-627 | ||
| 005 | 20240307060240.0 | ||
| 007 | cr uuu---uuuuu | ||
| 008 | 230823s2023 xx |||||o 00| ||eng c | ||
| 024 | 7 | |a 10.1038/s41467-023-38008-4 |2 doi | |
| 035 | |a (DE-627)185765305X | ||
| 035 | |a (DE-599)KXP185765305X | ||
| 035 | |a (OCoLC)1425212714 | ||
| 040 | |a DE-627 |b ger |c DE-627 |e rda | ||
| 041 | |a eng | ||
| 084 | |a 30 |2 sdnb | ||
| 100 | 1 | |a Jagt, Robert |e VerfasserIn |0 (DE-588)1310933618 |0 (DE-627)1871016924 |4 aut | |
| 245 | 1 | 0 | |a Layered BiOI single crystals capable of detecting low dose rates of X-rays |c Robert A. Jagt, Ivona Bravić, Lissa Eyre, Krzysztof Gałkowski, Joanna Borowiec, Kavya Reddy Dudipala, Michał Baranowski, Mateusz Dyksik, Tim W.J. van de Goor, Theo Kreouzis, Ming Xiao, Adrian Bevan, Paulina Płochocka, Samuel D. Stranks, Felix Deschler, Bartomeu Monserrat, Judith L. MacManus-Driscoll & Robert L.Z. Hoye |
| 264 | 1 | |c 28 April 2023 | |
| 300 | |b Illustrationen | ||
| 300 | |a 12 | ||
| 336 | |a Text |b txt |2 rdacontent | ||
| 337 | |a Computermedien |b c |2 rdamedia | ||
| 338 | |a Online-Ressource |b cr |2 rdacarrier | ||
| 500 | |a Gesehen am 23.11.2023 | ||
| 520 | |a Detecting low dose rates of X-rays is critical for making safer radiology instruments, but is limited by the absorber materials available. Here, we develop bismuth oxyiodide (BiOI) single crystals into effective X-ray detectors. BiOI features complex lattice dynamics, owing to the ionic character of the lattice and weak van der Waals interactions between layers. Through use of ultrafast spectroscopy, first-principles computations and detailed optical and structural characterisation, we show that photoexcited charge-carriers in BiOI couple to intralayer breathing phonon modes, forming large polarons, thus enabling longer drift lengths for the photoexcited carriers than would be expected if self-trapping occurred. This, combined with the low and stable dark currents and high linear X-ray attenuation coefficients, leads to strong detector performance. High sensitivities reaching 1.1 × 103 μC Gyair−1 cm−2 are achieved, and the lowest dose rate directly measured by the detectors was 22 nGyair s−1. The photophysical principles discussed herein offer new design avenues for novel materials with heavy elements and low-dimensional electronic structures for (opto)electronic applications. | ||
| 650 | 4 | |a Electronic devices | |
| 650 | 4 | |a Electronic properties and materials | |
| 700 | 1 | |a Bravić, Ivona |e VerfasserIn |4 aut | |
| 700 | 1 | |a Eyre, Lissa |e VerfasserIn |4 aut | |
| 700 | 1 | |a Gałkowski, Krzysztof |e VerfasserIn |4 aut | |
| 700 | 1 | |a Borowiec, Joanna |e VerfasserIn |4 aut | |
| 700 | 1 | |a Dudipala, Kavya Reddy |e VerfasserIn |4 aut | |
| 700 | 1 | |a Baranowski, Michał |e VerfasserIn |4 aut | |
| 700 | 1 | |a Dyksik, Mateusz |e VerfasserIn |4 aut | |
| 700 | 1 | |a van de Goor, Tim W. J. |e VerfasserIn |4 aut | |
| 700 | 1 | |a Kreouzis, Theo |e VerfasserIn |4 aut | |
| 700 | 1 | |a Xiao, Ming |e VerfasserIn |4 aut | |
| 700 | 1 | |a Bevan, Adrian |e VerfasserIn |4 aut | |
| 700 | 1 | |a Płochocka, Paulina |e VerfasserIn |4 aut | |
| 700 | 1 | |a Stranks, Samuel D. |e VerfasserIn |4 aut | |
| 700 | 1 | |a Deschler, Felix |e VerfasserIn |0 (DE-588)1266435395 |0 (DE-627)1815219386 |4 aut | |
| 700 | 1 | |a Monserrat, Bartomeu |e VerfasserIn |4 aut | |
| 700 | 1 | |a MacManus-Driscoll, Judith L. |e VerfasserIn |4 aut | |
| 700 | 1 | |a Hoye, Robert L. Z. |e VerfasserIn |4 aut | |
| 773 | 0 | 8 | |i Enthalten in |t Nature Communications |d [London] : Springer Nature, 2010 |g 14(2023), Artikel-ID 2452, Seite 1-12 |h Online-Ressource |w (DE-627)626457688 |w (DE-600)2553671-0 |w (DE-576)331555905 |x 2041-1723 |7 nnas |a Layered BiOI single crystals capable of detecting low dose rates of X-rays |
| 773 | 1 | 8 | |g volume:14 |g year:2023 |g elocationid:2452 |g pages:1-12 |g extent:12 |a Layered BiOI single crystals capable of detecting low dose rates of X-rays |
| 856 | 4 | 0 | |u https://doi.org/10.1038/s41467-023-38008-4 |x Verlag |x Resolving-System |z kostenfrei |3 Volltext |
| 856 | 4 | 0 | |u https://www.nature.com/articles/s41467-023-38008-4 |x Verlag |z kostenfrei |3 Volltext |
| 951 | |a AR | ||
| 992 | |a 20230823 | ||
| 993 | |a Article | ||
| 994 | |a 2023 | ||
| 998 | |g 1266435395 |a Deschler, Felix |m 1266435395:Deschler, Felix |d 120000 |d 120300 |e 120000PD1266435395 |e 120300PD1266435395 |k 0/120000/ |k 1/120000/120300/ |p 15 | ||
| 999 | |a KXP-PPN185765305X |e 4369572371 | ||
| BIB | |a Y | ||
| SER | |a journal | ||
| JSO | |a {"recId":"185765305X","relHost":[{"physDesc":[{"extent":"Online-Ressource"}],"disp":"Layered BiOI single crystals capable of detecting low dose rates of X-raysNature Communications","part":{"volume":"14","extent":"12","text":"14(2023), Artikel-ID 2452, Seite 1-12","year":"2023","pages":"1-12"},"title":[{"title":"Nature Communications","title_sort":"Nature Communications"}],"type":{"bibl":"periodical","media":"Online-Ressource"},"recId":"626457688","pubHistory":["2010-"],"origin":[{"publisherPlace":"[London] ; [London]","dateIssuedDisp":"[2010]-","publisher":"Springer Nature ; Nature Publishing Group UK"}],"note":["Gesehen am 13.06.24"],"id":{"zdb":["2553671-0"],"eki":["626457688"],"issn":["2041-1723"]},"language":["eng"]}],"note":["Gesehen am 23.11.2023"],"origin":[{"dateIssuedKey":"2023","dateIssuedDisp":"28 April 2023"}],"title":[{"title":"Layered BiOI single crystals capable of detecting low dose rates of X-rays","title_sort":"Layered BiOI single crystals capable of detecting low dose rates of X-rays"}],"person":[{"display":"Jagt, Robert","given":"Robert","role":"aut","family":"Jagt"},{"given":"Ivona","display":"Bravić, Ivona","role":"aut","family":"Bravić"},{"family":"Eyre","role":"aut","given":"Lissa","display":"Eyre, Lissa"},{"role":"aut","given":"Krzysztof","display":"Gałkowski, Krzysztof","family":"Gałkowski"},{"display":"Borowiec, Joanna","given":"Joanna","role":"aut","family":"Borowiec"},{"family":"Dudipala","display":"Dudipala, Kavya Reddy","given":"Kavya Reddy","role":"aut"},{"family":"Baranowski","role":"aut","given":"Michał","display":"Baranowski, Michał"},{"given":"Mateusz","display":"Dyksik, Mateusz","role":"aut","family":"Dyksik"},{"family":"van de Goor","given":"Tim W. J.","display":"van de Goor, Tim W. J.","role":"aut"},{"display":"Kreouzis, Theo","given":"Theo","role":"aut","family":"Kreouzis"},{"role":"aut","given":"Ming","display":"Xiao, Ming","family":"Xiao"},{"given":"Adrian","display":"Bevan, Adrian","role":"aut","family":"Bevan"},{"family":"Płochocka","role":"aut","given":"Paulina","display":"Płochocka, Paulina"},{"family":"Stranks","role":"aut","display":"Stranks, Samuel D.","given":"Samuel D."},{"given":"Felix","display":"Deschler, Felix","role":"aut","family":"Deschler"},{"display":"Monserrat, Bartomeu","given":"Bartomeu","role":"aut","family":"Monserrat"},{"family":"MacManus-Driscoll","display":"MacManus-Driscoll, Judith L.","given":"Judith L.","role":"aut"},{"role":"aut","given":"Robert L. Z.","display":"Hoye, Robert L. Z.","family":"Hoye"}],"id":{"eki":["185765305X"],"doi":["10.1038/s41467-023-38008-4"]},"physDesc":[{"extent":"12 S.","noteIll":"Illustrationen"}],"type":{"bibl":"article-journal","media":"Online-Ressource"},"language":["eng"],"name":{"displayForm":["Robert A. Jagt, Ivona Bravić, Lissa Eyre, Krzysztof Gałkowski, Joanna Borowiec, Kavya Reddy Dudipala, Michał Baranowski, Mateusz Dyksik, Tim W.J. van de Goor, Theo Kreouzis, Ming Xiao, Adrian Bevan, Paulina Płochocka, Samuel D. Stranks, Felix Deschler, Bartomeu Monserrat, Judith L. MacManus-Driscoll & Robert L.Z. Hoye"]}} | ||
| SRT | |a JAGTROBERTLAYEREDBIO2820 | ||