Phosphonite ligand design for nickel-catalyzed 2-methyl-3-butenenitrile isomerization and styrene hydrocyanation
The synthesis of a series of novel chelating bisphosphonite ligands with a bridged dihydroanthracene scaffold is described. First-generation derivatives showed a strong tendency for the formation of catalytically inactive Ni0 bis-chelate complexes. The solid state structures of these complexes allow...
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| Main Authors: | , , , , , |
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| Format: | Article (Journal) |
| Language: | English |
| Published: |
07 June 2010
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| In: |
ChemCatChem
Year: 2010, Volume: 2, Issue: 6, Pages: 674-682 |
| ISSN: | 1867-3899 |
| DOI: | 10.1002/cctc.201000022 |
| Online Access: | Verlag, lizenzpflichtig, Volltext: https://doi.org/10.1002/cctc.201000022 Verlag, lizenzpflichtig, Volltext: https://onlinelibrary.wiley.com/doi/abs/10.1002/cctc.201000022 
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| Author Notes: | Michael E. Tauchert, Thilo R. Kaiser, Alexander P.V. Göthlich, Frank Rominger, Daniel C.M. Warth, and Peter Hofmann |
MARC
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| 245 | 1 | 0 | |a Phosphonite ligand design for nickel-catalyzed 2-methyl-3-butenenitrile isomerization and styrene hydrocyanation |c Michael E. Tauchert, Thilo R. Kaiser, Alexander P.V. Göthlich, Frank Rominger, Daniel C.M. Warth, and Peter Hofmann |
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| 520 | |a The synthesis of a series of novel chelating bisphosphonite ligands with a bridged dihydroanthracene scaffold is described. First-generation derivatives showed a strong tendency for the formation of catalytically inactive Ni0 bis-chelate complexes. The solid state structures of these complexes allowed the design of tailor-made second-generation ligands for nickel-catalyzed 2-methyl-3-butenenitrile isomerization with exceptionally high activity. The second-generation catalyst also showed good catalytic performance in the hydrocyanation of styrene. | ||
| 650 | 4 | |a homogeneous catalysis | |
| 650 | 4 | |a hydrocyanation | |
| 650 | 4 | |a isomerization | |
| 650 | 4 | |a ligand design | |
| 650 | 4 | |a nickel | |
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