Observation of nuclear wave-packet interference in ultrafast interatomic energy transfer
We report the experimental observation of quantum interference in the nuclear wave-packet dynamics driving ultrafast excitation-energy transfer in argon dimers below the threshold of interatomic Coulombic decay (ICD). Using time-resolved photoion-photoion coincidence spectroscopy and quantum dynamic...
Saved in:
| Main Authors: | , , , , , |
|---|---|
| Format: | Article (Journal) |
| Language: | English |
| Published: |
23 June 2023
|
| In: |
Physical review letters
Year: 2023, Volume: 130, Issue: 25, Pages: 1-6 |
| ISSN: | 1079-7114 |
| DOI: | 10.1103/PhysRevLett.130.253202 |
| Online Access: | Verlag, lizenzpflichtig, Volltext: https://doi.org/10.1103/PhysRevLett.130.253202 Verlag, lizenzpflichtig, Volltext: https://link.aps.org/doi/10.1103/PhysRevLett.130.253202 
|
| Author Notes: | Meng Han, Jacqueline Fedyk, Jia-Bao Ji, Victor Despré, Alexander I. Kuleff, and Hans Jakob Wörner |
MARC
| LEADER | 00000caa a2200000 c 4500 | ||
|---|---|---|---|
| 001 | 1860924328 | ||
| 003 | DE-627 | ||
| 005 | 20240307051643.0 | ||
| 007 | cr uuu---uuuuu | ||
| 008 | 231009s2023 xx |||||o 00| ||eng c | ||
| 024 | 7 | |a 10.1103/PhysRevLett.130.253202 |2 doi | |
| 035 | |a (DE-627)1860924328 | ||
| 035 | |a (DE-599)KXP1860924328 | ||
| 035 | |a (OCoLC)1425210832 | ||
| 040 | |a DE-627 |b ger |c DE-627 |e rda | ||
| 041 | |a eng | ||
| 084 | |a 30 |2 sdnb | ||
| 100 | 1 | |a Han, Meng |d 1972- |e VerfasserIn |0 (DE-588)123710804 |0 (DE-627)706403738 |0 (DE-576)293838801 |4 aut | |
| 245 | 1 | 0 | |a Observation of nuclear wave-packet interference in ultrafast interatomic energy transfer |c Meng Han, Jacqueline Fedyk, Jia-Bao Ji, Victor Despré, Alexander I. Kuleff, and Hans Jakob Wörner |
| 264 | 1 | |c 23 June 2023 | |
| 300 | |b Illustrationen | ||
| 300 | |a 6 | ||
| 336 | |a Text |b txt |2 rdacontent | ||
| 337 | |a Computermedien |b c |2 rdamedia | ||
| 338 | |a Online-Ressource |b cr |2 rdacarrier | ||
| 500 | |a Gesehen am 06.12.2023 | ||
| 520 | |a We report the experimental observation of quantum interference in the nuclear wave-packet dynamics driving ultrafast excitation-energy transfer in argon dimers below the threshold of interatomic Coulombic decay (ICD). Using time-resolved photoion-photoion coincidence spectroscopy and quantum dynamics simulations, we reveal that the electronic relaxation dynamics of the inner-valence 3s hole on one atom leading to a 4s or 4p excitation on the other one is influenced by nuclear quantum dynamics in the initial state, giving rise to a deep, periodic modulation on the kinetic-energy-release (KER) spectra of the coincident Ar+−Ar+ ion pairs. Moreover, the time-resolved KER spectra show characteristic fingerprints of quantum interference effects during the energy-transfer process. Our findings pave the way to elucidating quantum-interference effects in ultrafast charge- and energy-transfer dynamics in more complex systems, such as molecular clusters and solvated molecules. | ||
| 700 | 1 | |a Fedyk, Jacqueline |d 1994- |e VerfasserIn |0 (DE-588)1209133318 |0 (DE-627)1696279046 |4 aut | |
| 700 | 1 | |a Ji, Jia-Bao |e VerfasserIn |4 aut | |
| 700 | 1 | |a Despré, Victor |e VerfasserIn |0 (DE-588)1160946256 |0 (DE-627)1024327329 |0 (DE-576)506264629 |4 aut | |
| 700 | 1 | |a Kuleff, Alexander I. |d 1973- |e VerfasserIn |0 (DE-588)1148996362 |0 (DE-627)1009297600 |0 (DE-576)496511327 |4 aut | |
| 700 | 1 | |a Wörner, Hans Jakob |d 1981- |e VerfasserIn |0 (DE-588)1089593260 |0 (DE-627)853375542 |0 (DE-576)460018361 |4 aut | |
| 773 | 0 | 8 | |i Enthalten in |t Physical review letters |d College Park, Md. : APS, 1958 |g 130(2023), 25 vom: Juni, Artikel-ID 253202, Seite 1-6 |h Online-Ressource |w (DE-627)268756899 |w (DE-600)1472655-5 |w (DE-576)077609441 |x 1079-7114 |7 nnas |a Observation of nuclear wave-packet interference in ultrafast interatomic energy transfer |
| 773 | 1 | 8 | |g volume:130 |g year:2023 |g number:25 |g month:06 |g elocationid:253202 |g pages:1-6 |g extent:6 |a Observation of nuclear wave-packet interference in ultrafast interatomic energy transfer |
| 856 | 4 | 0 | |u https://doi.org/10.1103/PhysRevLett.130.253202 |x Verlag |x Resolving-System |z lizenzpflichtig |3 Volltext |
| 856 | 4 | 0 | |u https://link.aps.org/doi/10.1103/PhysRevLett.130.253202 |x Verlag |z lizenzpflichtig |3 Volltext |
| 951 | |a AR | ||
| 992 | |a 20231009 | ||
| 993 | |a Article | ||
| 994 | |a 2023 | ||
| 998 | |g 1148996362 |a Kuleff, Alexander I. |m 1148996362:Kuleff, Alexander I. |d 120000 |d 120300 |e 120000PK1148996362 |e 120300PK1148996362 |k 0/120000/ |k 1/120000/120300/ |p 5 | ||
| 998 | |g 1160946256 |a Despré, Victor |m 1160946256:Despré, Victor |d 120000 |d 120300 |e 120000PD1160946256 |e 120300PD1160946256 |k 0/120000/ |k 1/120000/120300/ |p 4 | ||
| 998 | |g 1209133318 |a Fedyk, Jacqueline |m 1209133318:Fedyk, Jacqueline |d 120000 |d 120300 |e 120000PF1209133318 |e 120300PF1209133318 |k 0/120000/ |k 1/120000/120300/ |p 2 | ||
| 999 | |a KXP-PPN1860924328 |e 4382665892 | ||
| BIB | |a Y | ||
| SER | |a journal | ||
| JSO | |a {"person":[{"role":"aut","roleDisplay":"VerfasserIn","display":"Han, Meng","given":"Meng","family":"Han"},{"display":"Fedyk, Jacqueline","roleDisplay":"VerfasserIn","role":"aut","family":"Fedyk","given":"Jacqueline"},{"display":"Ji, Jia-Bao","roleDisplay":"VerfasserIn","role":"aut","family":"Ji","given":"Jia-Bao"},{"family":"Despré","given":"Victor","roleDisplay":"VerfasserIn","display":"Despré, Victor","role":"aut"},{"role":"aut","display":"Kuleff, Alexander I.","roleDisplay":"VerfasserIn","given":"Alexander I.","family":"Kuleff"},{"role":"aut","display":"Wörner, Hans Jakob","roleDisplay":"VerfasserIn","given":"Hans Jakob","family":"Wörner"}],"title":[{"title":"Observation of nuclear wave-packet interference in ultrafast interatomic energy transfer","title_sort":"Observation of nuclear wave-packet interference in ultrafast interatomic energy transfer"}],"language":["eng"],"recId":"1860924328","note":["Gesehen am 06.12.2023"],"type":{"bibl":"article-journal","media":"Online-Ressource"},"name":{"displayForm":["Meng Han, Jacqueline Fedyk, Jia-Bao Ji, Victor Despré, Alexander I. Kuleff, and Hans Jakob Wörner"]},"id":{"eki":["1860924328"],"doi":["10.1103/PhysRevLett.130.253202"]},"origin":[{"dateIssuedKey":"2023","dateIssuedDisp":"23 June 2023"}],"relHost":[{"pubHistory":["1.1958 -"],"part":{"year":"2023","pages":"1-6","issue":"25","volume":"130","text":"130(2023), 25 vom: Juni, Artikel-ID 253202, Seite 1-6","extent":"6"},"titleAlt":[{"title":"Physical review letters online"},{"title":"Physical review L"}],"disp":"Observation of nuclear wave-packet interference in ultrafast interatomic energy transferPhysical review letters","type":{"bibl":"periodical","media":"Online-Ressource"},"note":["Gesehen am 23.08.2019"],"corporate":[{"role":"isb","display":"American Physical Society","roleDisplay":"Herausgebendes Organ"}],"language":["eng"],"recId":"268756899","title":[{"title_sort":"Physical review letters","title":"Physical review letters"}],"physDesc":[{"extent":"Online-Ressource"}],"origin":[{"dateIssuedDisp":"1958-","dateIssuedKey":"1958","publisher":"APS","publisherPlace":"College Park, Md."}],"id":{"issn":["1079-7114"],"zdb":["1472655-5"],"eki":["268756899"]},"name":{"displayForm":["publ. by the American Physical Society"]}}],"physDesc":[{"extent":"6 S.","noteIll":"Illustrationen"}]} | ||
| SRT | |a HANMENGFEDOBSERVATIO2320 | ||